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More water\u2010rich networks are typically less mechanically robust, which is manifested as softness and low stress to fracture. Unusually, jellyfish mesoglea exhibits paradoxical combination of high stiffness and strength with ultrahigh water content. Here, it is discovered that jellyfish mesoglea possesses a long\u2010range\u2010ordered laminated membranous network, which features crystal orientation along membrane plane and collagen chain spanning at the junction of membranes. Such a laminated membranous network is in favor of resistance to deformation, as well as transmission and dispersion of stress for culminating in good mechanical robustness. Fabrication of chitosan hydrogel with jellyfish mesoglea\u2010like network is further demonstrated by pre\u2010constructing a random membranous network via evaporation\u2010induced phase separation, followed by aligning and crystallizing the membranes via combination of in\u2010plane stretching and sodium hydroxide treatment. The obtained hydrogel exhibits a combination of high modulus (5.2\u00a0MPa) and strength (6.5\u00a0MPa) with ultrahigh water content (91.8\u00a0wt.%), exceeding that of other synthetic and even biological hydrogels. This work offers not only a structural concept but also a feasible way for making hydrogels that overcome traditional trade\u2010off between good mechanical robustness and ultrahigh water content.<\/jats:p>","DOI":"10.1002\/adma.202511595","type":"journal-article","created":{"date-parts":[[2025,10,13]],"date-time":"2025-10-13T07:34:47Z","timestamp":1760340887000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":14,"title":["Ultrahigh\u2010Water\u2010Content yet Robust Hydrogels Enabled by Bioinspired Laminated Membranous Network"],"prefix":"10.1002","volume":"38","author":[{"given":"Shunxi","family":"Wen","sequence":"first","affiliation":[{"name":"College of Materials Science and Engineering Hunan Province Key Laboratory of Bioinspired Polymer Materials Hunan University  Changsha 410082 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