{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,9,4]],"date-time":"2026-09-04T22:02:41Z","timestamp":1788559361135,"version":"build-2803163510"},"reference-count":61,"publisher":"Wiley","issue":"1","license":[{"start":{"date-parts":[[2025,9,18]],"date-time":"2025-09-18T00:00:00Z","timestamp":1758153600000},"content-version":"vor","delay-in-days":0,"URL":"http:\/\/onlinelibrary.wiley.com\/termsAndConditions#vor"}],"funder":[{"DOI":"10.13039\/501100005090","name":"Beijing Nova Program","doi-asserted-by":"publisher","award":["20240484638"],"award-info":[{"award-number":["20240484638"]}],"id":[{"id":"10.13039\/501100005090","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["52070006"],"award-info":[{"award-number":["52070006"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":["advanced.onlinelibrary.wiley.com"],"crossmark-restriction":true},"short-container-title":["Advanced Materials"],"published-print":{"date-parts":[[2026,1]]},"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>\n                    In the field of gas phase catalysis, reactive oxygen species (ROS) play a crucial role, but how to improve catalytic efficiency and lifetime by forming ROS efficiently and sustainably during the catalytic process is a challenge for high\u2010performance catalysts. Here, a pyroelectric enhanced catalytic oxidation (PECO) strategy is reported that can effectively enhance the catalytic oxidation efficiency and life of the catalyst by constantly generation of ROS. When gaseous pollutants of formaldehyde (HCHO) are catalytically degraded by conductive aerogel catalysts of MnO\n                    <jats:italic>\n                      <jats:sub>x<\/jats:sub>\n                    <\/jats:italic>\n                    , the HCHO to CO\n                    <jats:sub>2<\/jats:sub>\n                    conversion efficiency is increased by \u2248300% to 95.33% at a high gas hourly space velocity (GHSV: 600 L\u00a0g\n                    <jats:sub>cat.<\/jats:sub>\n                    <jats:sup>\u22121<\/jats:sup>\n                    \u00b7h\n                    <jats:sup>\u22121<\/jats:sup>\n                    ) using the pyroelectric effect of BaTiO\n                    <jats:sub>3<\/jats:sub>\n                    , and the efficiency attenuation is less than 3% during the continuous catalytic process of 1200\u00a0h. The experimental and theoretical analysis confirm that the pyroelectric effect contributes to improving valence transition of Mn\n                    <jats:sup>3+<\/jats:sup>\n                    \/Mn\n                    <jats:sup>4+<\/jats:sup>\n                    and electron transfer of oxygen\u2010containing molecules thus leading to the continuous formation of ROS. The PECO strategy provides a simple and effective approach for ROS engineering and has broad application prospects in the field of catalysis.\n                  <\/jats:p>","DOI":"10.1002\/adma.202512417","type":"journal-article","created":{"date-parts":[[2025,9,18]],"date-time":"2025-09-18T10:01:04Z","timestamp":1758189664000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":6,"title":["Pyroelectric Enhanced Catalytic Oxidation: A Universal Strategy for Low\u2010Temperature Gas Phase Catalysis"],"prefix":"10.1002","volume":"38","author":[{"given":"De Cai","family":"Fang","sequence":"first","affiliation":[{"name":"Key Laboratory of Advanced Functional Materials, Ministry of Education College of Materials Science and Engineering State Key Laboratory of Materials Low\u2010Carbon Recycling Beijing University of Technology Beijing 100124 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zi Qiang","family":"Ma","sequence":"additional","affiliation":[{"name":"Key Laboratory of Advanced Functional Materials, Ministry of Education College of Materials Science and Engineering State Key Laboratory of Materials Low\u2010Carbon Recycling Beijing University of Technology Beijing 100124 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Li Hong","family":"Chang","sequence":"additional","affiliation":[{"name":"Key Laboratory of Advanced Functional Materials, Ministry of Education College of Materials Science and Engineering State Key Laboratory of Materials Low\u2010Carbon Recycling Beijing University of Technology Beijing 100124 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-2521-8033","authenticated-orcid":false,"given":"Chang Bao","family":"Han","sequence":"additional","affiliation":[{"name":"Key Laboratory of Advanced Functional Materials, Ministry of Education College of Materials Science and Engineering State Key Laboratory of Materials Low\u2010Carbon Recycling Beijing University of Technology Beijing 100124 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Hui","family":"Yan","sequence":"additional","affiliation":[{"name":"Key Laboratory of Advanced Functional Materials, Ministry of Education College of Materials Science and Engineering State Key Laboratory of Materials Low\u2010Carbon Recycling Beijing University of Technology Beijing 100124 China"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2025,9,18]]},"reference":[{"key":"e_1_2_8_1_1","doi-asserted-by":"publisher","DOI":"10.1021\/jacs.4c02531"},{"key":"e_1_2_8_1_2","doi-asserted-by":"publisher","DOI":"10.1038\/s41929-023-01090-4"},{"key":"e_1_2_8_1_3","doi-asserted-by":"publisher","DOI":"10.1038\/s41929-023-01027-x"},{"key":"e_1_2_8_2_1","doi-asserted-by":"publisher","DOI":"10.1021\/acscatal.3c05978"},{"key":"e_1_2_8_3_1","doi-asserted-by":"publisher","DOI":"10.1021\/acs.est.4c05249"},{"key":"e_1_2_8_4_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.apcatb.2024.124912"},{"key":"e_1_2_8_5_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.jhazmat.2024.133613"},{"key":"e_1_2_8_5_2","doi-asserted-by":"publisher","DOI":"10.1038\/s41467-020-16119-6"},{"key":"e_1_2_8_6_1","doi-asserted-by":"publisher","DOI":"10.1021\/acs.est.2c09861"},{"key":"e_1_2_8_7_1","doi-asserted-by":"publisher","DOI":"10.1021\/acscatal.4c00863"},{"key":"e_1_2_8_7_2","doi-asserted-by":"publisher","DOI":"10.1038\/s41467-021-27789-1"},{"key":"e_1_2_8_7_3","doi-asserted-by":"publisher","DOI":"10.1016\/j.apcatb.2024.124139"},{"key":"e_1_2_8_8_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41929-021-00702-1"},{"key":"e_1_2_8_9_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.apcatb.2024.123828"},{"key":"e_1_2_8_9_2","doi-asserted-by":"publisher","DOI":"10.1021\/acs.est.0c03981"},{"key":"e_1_2_8_10_1","doi-asserted-by":"publisher","DOI":"10.1039\/D3CS00213F"},{"key":"e_1_2_8_11_1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.202313661"},{"key":"e_1_2_8_12_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.chemosphere.2018.06.064"},{"key":"e_1_2_8_13_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.cej.2024.158291"},{"key":"e_1_2_8_14_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41560-024-01541-7"},{"key":"e_1_2_8_15_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41467-020-20517-1"},{"key":"e_1_2_8_16_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.joule.2023.12.006"},{"key":"e_1_2_8_16_2","doi-asserted-by":"publisher","DOI":"10.1002\/smll.202103960"},{"key":"e_1_2_8_17_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41467-022-33818-4"},{"key":"e_1_2_8_17_2","doi-asserted-by":"publisher","DOI":"10.1016\/j.nanoen.2020.105371"},{"key":"e_1_2_8_17_3","doi-asserted-by":"publisher","DOI":"10.1038\/s41467-025-57672-2"},{"key":"e_1_2_8_17_4","doi-asserted-by":"publisher","DOI":"10.1038\/s41467-023-40954-y"},{"key":"e_1_2_8_17_5","doi-asserted-by":"publisher","DOI":"10.1002\/adma.202207391"},{"key":"e_1_2_8_18_1","doi-asserted-by":"publisher","DOI":"10.1039\/C6NR00972G"},{"key":"e_1_2_8_19_1","doi-asserted-by":"publisher","DOI":"10.1002\/aenm.202401739"},{"key":"e_1_2_8_20_1","doi-asserted-by":"publisher","DOI":"10.1002\/adfm.202302360"},{"key":"e_1_2_8_21_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.nanoen.2020.104448"},{"key":"e_1_2_8_22_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.gee.2022.01.008"},{"key":"e_1_2_8_23_1","doi-asserted-by":"publisher","DOI":"10.1021\/jacs.3c11847"},{"key":"e_1_2_8_23_2","doi-asserted-by":"publisher","DOI":"10.1016\/j.cej.2018.06.128"},{"key":"e_1_2_8_24_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41467-025-59081-x"},{"key":"e_1_2_8_25_1","doi-asserted-by":"publisher","DOI":"10.1021\/acscatal.9b04637"},{"key":"e_1_2_8_26_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.jhazmat.2024.134382"},{"key":"e_1_2_8_27_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.apcatb.2025.125036"},{"key":"e_1_2_8_27_2","doi-asserted-by":"publisher","DOI":"10.1021\/acscatal.4c04284"},{"key":"e_1_2_8_27_3","doi-asserted-by":"publisher","DOI":"10.1002\/adfm.202401281"},{"key":"e_1_2_8_28_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.apcatb.2024.124253"},{"key":"e_1_2_8_29_1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.201905823"},{"key":"e_1_2_8_30_1","doi-asserted-by":"publisher","DOI":"10.1039\/C8CS00583D"},{"key":"e_1_2_8_31_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.cej.2020.125790"},{"key":"e_1_2_8_32_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41929-024-01175-8"},{"key":"e_1_2_8_33_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.apcatb.2023.122837"},{"key":"e_1_2_8_34_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.apcatb.2024.124169"},{"key":"e_1_2_8_35_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.apcatb.2016.05.058"},{"key":"e_1_2_8_36_1","doi-asserted-by":"publisher","DOI":"10.1063\/1.4812323"},{"key":"e_1_2_8_37_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.watres.2024.123027"},{"key":"e_1_2_8_37_2","doi-asserted-by":"publisher","DOI":"10.1016\/j.apcatb.2024.124099"},{"key":"e_1_2_8_38_1","doi-asserted-by":"publisher","DOI":"10.1021\/acscatal.4c07213"},{"key":"e_1_2_8_39_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41467-021-21055-0"},{"key":"e_1_2_8_40_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41563-025-02171-4"},{"key":"e_1_2_8_41_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.apcatb.2020.119294"},{"key":"e_1_2_8_41_2","doi-asserted-by":"publisher","DOI":"10.1016\/j.cej.2022.138147"},{"key":"e_1_2_8_42_1","doi-asserted-by":"publisher","DOI":"10.1002\/aenm.201400519"},{"key":"e_1_2_8_43_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.joule.2024.09.009"},{"key":"e_1_2_8_44_1","doi-asserted-by":"publisher","DOI":"10.1002\/advs.202105368"},{"key":"e_1_2_8_45_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41467-022-32132-3"}],"container-title":["Advanced Materials"],"original-title":[],"language":"en","link":[{"URL":"https:\/\/advanced.onlinelibrary.wiley.com\/doi\/pdf\/10.1002\/adma.202512417","content-type":"unspecified","content-version":"vor","intended-application":"similarity-checking"}],"deposited":{"date-parts":[[2026,1,3]],"date-time":"2026-01-03T06:29:20Z","timestamp":1767421760000},"score":1,"resource":{"primary":{"URL":"https:\/\/advanced.onlinelibrary.wiley.com\/doi\/10.1002\/adma.202512417"}},"subtitle":[],"short-title":[],"issued":{"date-parts":[[2025,9,18]]},"references-count":61,"journal-issue":{"issue":"1","published-print":{"date-parts":[[2026,1]]}},"alternative-id":["10.1002\/adma.202512417"],"URL":"https:\/\/doi.org\/10.1002\/adma.202512417","archive":["Portico"],"relation":{},"ISSN":["0935-9648","1521-4095"],"issn-type":[{"value":"0935-9648","type":"print"},{"value":"1521-4095","type":"electronic"}],"subject":[],"published":{"date-parts":[[2025,9,18]]},"assertion":[{"value":"2025-06-30","order":0,"name":"received","label":"Received","group":{"name":"publication_history","label":"Publication History"}},{"value":"2025-09-18","order":3,"name":"published","label":"Published","group":{"name":"publication_history","label":"Publication History"}}],"article-number":"e12417"}}