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Their performance depends on high ionic conductivity, chemical\/physical stability, and scalable manufacture of solid electrolytes (SEs). This study compares sulfide\u2010 and halide\u2010based SEs, two promising next\u2010generation energy storage options. Soft mechanics permit sulfides with high room\u2010temperature conductivity, low activation energies, and processability, but high\u2010voltage cathode instability, moisture sensitivity, and probable hydrogen sulfide (H\n                    <jats:sub>2<\/jats:sub>\n                    S) release. Market prospects are favorable as the industry improves crystallinity and elemental substitution, especially for automotive cells. Chloride\u2010based halides are more environmentally friendly, have adequate voltage stability, and can be used with oxide cathodes without coatings. Despite traditionally low conductivity, high\u2010entropy, and oxyhalide chemistries currently reach 10 mS cm\n                    <jats:sup>\u22121<\/jats:sup>\n                    , and scalable solvent syntheses and dry processing are driving adoption. Mechanical compliance and the use of rare elements (In, Sc) continue to cause integration and cost issues. Composition, microstructure, synthesis techniques, interfacial behavior, mechanical characteristics, and scalability are evaluated. The findings show sulfides have better conductivity and Li\u2010metal compatibility, but halides are more stable and manufacturable, recommending hybrid or tailored material selection based on application. Optimizing ASSB systems requires complementary sulfide\/chloride utilization due to halides' mechanical constraints.\n                  <\/jats:p>","DOI":"10.1002\/adma.202513255","type":"journal-article","created":{"date-parts":[[2025,9,29]],"date-time":"2025-09-29T06:50:36Z","timestamp":1759128636000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":53,"title":["Comparative Advances in Sulfide and Halide Electrolytes for Commercialization of All\u2010Solid\u2010State Lithium Batteries"],"prefix":"10.1002","volume":"38","author":[{"given":"Mohamed Djihad","family":"Bouguern","sequence":"first","affiliation":[{"name":"Department of Chemical and Materials Engineering Concordia University  Montreal QC H3G 1M8 Canada"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0002-1239-8813","authenticated-orcid":false,"given":"Ningaraju Gejjiganahalli","family":"Ningappa","sequence":"additional","affiliation":[{"name":"Department of Chemical and Materials Engineering Concordia University  Montreal QC H3G 1M8 Canada"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0003-6085-9474","authenticated-orcid":false,"given":"Karthik","family":"Vishweswariah","sequence":"additional","affiliation":[{"name":"Department of Chemical and Materials Engineering Concordia University  Montreal QC H3G 1M8 Canada"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Anil","family":"Kumar M R","sequence":"additional","affiliation":[{"name":"Department of Chemical and Materials Engineering Concordia University  Montreal QC H3G 1M8 Canada"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-0593-2515","authenticated-orcid":false,"given":"Ryoji","family":"Kanno","sequence":"additional","affiliation":[{"name":"Research Center for All\u2010Solid\u2010State Battery Institute of Integrated Research Institute of Science Tokyo  4259 Nagatsuta Midori\u2010ku Yokohama 226\u20108502 Japan"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0006-9548-9989","authenticated-orcid":false,"given":"Karim","family":"Zaghib","sequence":"additional","affiliation":[{"name":"Department of Chemical and Materials Engineering Concordia University  Montreal QC H3G 1M8 Canada"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2025,9,28]]},"reference":[{"key":"e_1_2_8_1_1","doi-asserted-by":"publisher","DOI":"10.1179\/amb.1980.27.1.26"},{"key":"e_1_2_8_2_1","doi-asserted-by":"publisher","DOI":"10.1098\/rstl.1839.0002"},{"key":"e_1_2_8_3_1","doi-asserted-by":"publisher","DOI":"10.4271\/680453"},{"key":"e_1_2_8_4_1","first-page":"209","volume":"9","author":"Nagaura T.","year":"1990","journal-title":"Prog. 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