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However, their nanoscale dimensions \u2014 smaller than the mean free path of secondary carriers \u2014 and relatively low emitter density per unit volume, limited by their high molecular weight and reabsorption losses, restrict efficient secondary carrier conversion and hamper their practical deployment. In this work, a strategy is introduced to enhance scintillation performance by organizing NCs into densely packed domains within porous SiO\n                    <jats:sub>2<\/jats:sub>\n                    mesospheres (MSNs). This engineered architecture achieves up to a 40\u2010fold increase in radioluminescence intensity compared to colloidal NCs, driven by improved retention and conversion of secondary charges, as corroborated by electron release measurements. This approach offers a promising pathway toward developing next\u2010generation nanoscintillators with enhanced performance, with potential applications in high\u2010energy physics, medical imaging, and space technologies.\n                  <\/jats:p>","DOI":"10.1002\/adma.202513469","type":"journal-article","created":{"date-parts":[[2025,10,15]],"date-time":"2025-10-15T19:39:08Z","timestamp":1760557148000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":7,"title":["Harnessing Self\u2010Sensitized Scintillation by Supramolecular Engineering of CsPbBr\n                    <sub>3<\/sub>\n                    Nanocrystals in Dense Mesoporous Template Nanospheres"],"prefix":"10.1002","volume":"38","author":[{"ORCID":"https:\/\/orcid.org\/0000-0001-8995-7025","authenticated-orcid":false,"given":"Xiaohe","family":"Zhou","sequence":"first","affiliation":[{"name":"Dipartimento di Scienza dei Materiali Universit\u00e0 degli Studi di Milano\u2010Bicocca Via R. 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