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Nevertheless, the critical challenge of interfacial incompatibility between MOST molecules and fabrics persists, resulting in compromised robustness and suboptimal energy conversion efficiency. Here, inspired by the salt absorption\u2010secretion mechanism of\n                    <jats:italic>Atriplex centralasiatica<\/jats:italic>\n                    , an innovative swelling\u2010deswelling strategy tailored for hollow aerogel fibers (HAFs) is developed, creating a synergistically promoted MOST\u2010fabric system (SPMFS) with concurrent enhancements in mechanical robustness and photothermal performance. During the swelling\u2010deswelling process, thermoplastic polyurethane (TPU) chains undergo reorganization into a densified network, while the simultaneous secretion of azobenzene (Azo) forms dense, uniform monocrystalline layers. The resultant SPMFS exhibits notable mechanical improvements, with a 48% increase in breaking strain and 129% enhancement in tensile strength. Equally striking are its photothermal capabilities, achieving an enhanced photo\u2010charging and photo\u2010discharging (&gt;94% photoconversion) alongside a uniformly distributed high energy density of 7.5 kJ m\n                    <jats:sup>\u22122<\/jats:sup>\n                    . Moreover, the SPMFS enables programmable rapid thermal management, showcases impressive durability under long\u2010term washing, cyclic stretching, and rubbing, and realizes controllable photothermal physiotherapy. This bioinspired strategy lays the groundwork for next\u2010generation wearable PTM systems and establishes a framework for future PTM device design\n                  <\/jats:p>","DOI":"10.1002\/adma.202514043","type":"journal-article","created":{"date-parts":[[2025,10,6]],"date-time":"2025-10-06T23:25:48Z","timestamp":1759793148000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":18,"title":["Bioinspired Swelling\u2010Deswelling Strategy Unlocks Synergistic Molecular Solar Thermal\u2010Fabric Systems for Personal Thermal Management"],"prefix":"10.1002","volume":"38","author":[{"given":"Shuo","family":"Wang","sequence":"first","affiliation":[{"name":"School of Materials Science and Engineering and Tianjin Key Laboratory of Composite and Functional Materials Tianjin University  Tianjin 300350 P. R. 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