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Here, the first intrinsically ductile\/plastic inorganic ferromagnetic semiconductor, bulk CrSiTe\n                    <jats:sub>3<\/jats:sub>\n                    van der Waals (vdW) crystals, which combine excellent deformability with ferromagnetism, is reported. Mechanical characterization reveals excellent plasticity at room temperature, with CrSiTe\n                    <jats:sub>3<\/jats:sub>\n                    crystals sustaining up to 12% tensile strain, surpassing many existing plastic bulk vdW semiconductors. Below the Curie temperature of 34\u00a0K, the material retains ferromagnetic ordering, with plasticity exerting negligible effects on Curie temperature or saturation magnetization. First\u2010principles calculations attribute the exceptional deformability to low interlayer slip energy barriers and high cleavage energy within Te\u2010terminated vdW layers, enabling interlayer gliding without fracture. Monte Carlo simulations confirm that interlayer slip minimally perturbs magnetic interactions, preserving ferromagnetism. This work bridges the gap between mechanical plasticity, semiconductivity, and ferromagnetism in a single material, extending the functionality of plastic inorganic semiconductors.\n                  <\/jats:p>","DOI":"10.1002\/adma.202514083","type":"journal-article","created":{"date-parts":[[2025,10,7]],"date-time":"2025-10-07T12:24:21Z","timestamp":1759839861000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":6,"title":["Ductile Inorganic Ferromagnetic Semiconductor"],"prefix":"10.1002","volume":"38","author":[{"ORCID":"https:\/\/orcid.org\/0009-0008-0371-4347","authenticated-orcid":false,"given":"Jun","family":"Luo","sequence":"first","affiliation":[{"name":"State Key Laboratory of High Performance Ceramics, Shanghai Institute of Ceramics Chinese Academy of Sciences  Shanghai 200050 China"},{"name":"Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of Sciences  Beijing 100049 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-5182-3766","authenticated-orcid":false,"given":"Jun","family":"Chen","sequence":"additional","affiliation":[{"name":"Key Laboratory of Quantum Materials and Devices of Ministry of Education, School of Physics Southeast University  Nanjing 211189 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zhiqiang","family":"Gao","sequence":"additional","affiliation":[{"name":"State Key Laboratory of High Performance Ceramics, Shanghai Institute of Ceramics Chinese Academy of Sciences  Shanghai 200050 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jiali","family":"Zhou","sequence":"additional","affiliation":[{"name":"State Key Laboratory of High Performance Ceramics, Shanghai Institute of Ceramics Chinese Academy of Sciences  Shanghai 200050 China"},{"name":"Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of Sciences  Beijing 100049 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-0740-0851","authenticated-orcid":false,"given":"Jiawei","family":"Zhang","sequence":"additional","affiliation":[{"name":"State Key Laboratory of High Performance Ceramics, Shanghai Institute of Ceramics Chinese Academy of Sciences  Shanghai 200050 China"},{"name":"Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of Sciences  Beijing 100049 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Pengfei","family":"Qiu","sequence":"additional","affiliation":[{"name":"State Key Laboratory of High Performance Ceramics, Shanghai Institute of Ceramics Chinese Academy of Sciences  Shanghai 200050 China"},{"name":"Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of Sciences  Beijing 100049 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Shengchun","family":"Shen","sequence":"additional","affiliation":[{"name":"Hefei National Research Center for Physical Sciences at the Microscale, Department of Physics and CAS Key Laboratory of Strongly\u2010Coupled Quantum Matter Physics University of Science and Technology of China  Hefei 230026 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-6910-6319","authenticated-orcid":false,"given":"Shuai","family":"Dong","sequence":"additional","affiliation":[{"name":"Key Laboratory of Quantum Materials and Devices of Ministry of Education, School of Physics Southeast University  Nanjing 211189 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Lidong","family":"Chen","sequence":"additional","affiliation":[{"name":"State Key Laboratory of High Performance Ceramics, Shanghai Institute of Ceramics Chinese Academy of Sciences  Shanghai 200050 China"},{"name":"Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of Sciences  Beijing 100049 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-8086-6407","authenticated-orcid":false,"given":"Xun","family":"Shi","sequence":"additional","affiliation":[{"name":"State Key Laboratory of High Performance Ceramics, Shanghai Institute of Ceramics Chinese Academy of Sciences  Shanghai 200050 China"},{"name":"Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of Sciences  Beijing 100049 China"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2025,10,7]]},"reference":[{"key":"e_1_2_9_1_1","doi-asserted-by":"publisher","DOI":"10.1016\/0749-6419(87)90021-0"},{"key":"e_1_2_9_2_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.ijplas.2015.08.003"},{"key":"e_1_2_9_3_1","doi-asserted-by":"publisher","DOI":"10.1002\/idm2.12209"},{"key":"e_1_2_9_4_1","volume-title":"Semiconductors: Bonds and bands","author":"Ferry D. 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