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The greater degree of disorders in organic semiconductors, compared to inorganic semiconductors, is one of the major obstacles to their performance; thus, minimizing disorders is a key approach to boost the performance of organic electronics. Here, a strategy of using phthalate esters is introduced as assembly\u2010inducing agents (AIAs) to improve the packing ordering of organic semiconductors, thereby reducing the energetic disorders and improving the device performance. With dioctyl phthalate AIA, the organic semiconductor PM6 shows a 24% reduction in Urbach energy, 11% narrower absorption full width at half maximum, and suppressed absorption tails in thin film. In organic field\u2010effect transistors, this strategy offers a lift of hole mobility by 33.3%. In semitransparent organic photovoltaics, this strategy improves the average visible transmittance by 11.2% while maintaining the power conversion efficiency, yielding a high light utilization efficiency of 4.63% in optical structure\u2010free devices. This work provides a facile and effective approach to suppress the energetic disorder of organic semiconductors and opens up a new avenue for fabricating high\u2010performance organic electronics.<\/jats:p>","DOI":"10.1002\/adma.202515077","type":"journal-article","created":{"date-parts":[[2025,11,28]],"date-time":"2025-11-28T14:18:02Z","timestamp":1764339482000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":8,"title":["Suppressing Energetic Disorder of Organic Semiconductors for Semitransparent Photovoltaics and Thin\u2010Film Transistors"],"prefix":"10.1002","volume":"38","author":[{"given":"Yingyue","family":"Hu","sequence":"first","affiliation":[{"name":"College of Polymer Science and Engineering State Key Laboratory of Advanced Polymer Materials Sichuan University  Chengdu 610065 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-2509-4579","authenticated-orcid":false,"given":"Jiayu","family":"Wang","sequence":"additional","affiliation":[{"name":"College of Polymer Science and Engineering State Key Laboratory of Advanced Polymer Materials Sichuan University  Chengdu 610065 China"},{"name":"School of Materials Science and Engineering Peking University  Beijing 100871 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Hongxiang","family":"Li","sequence":"additional","affiliation":[{"name":"College of Polymer Science and Engineering State Key Laboratory of Advanced Polymer Materials Sichuan University  Chengdu 610065 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Si","family":"Chen","sequence":"additional","affiliation":[{"name":"KAUST Solar Center (KSC), Physical Science and Engineering Division (PSE), Material Science and Engineering Program (MSE) King Abdullah University of Science and Technology (KAUST)  Thuwal 23955\u20136900 Kingdom of Saudi Arabia"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Hua","family":"Tang","sequence":"additional","affiliation":[{"name":"KAUST Solar Center (KSC), Physical Science and Engineering Division (PSE), Material Science and Engineering Program (MSE) King Abdullah University of Science and Technology (KAUST)  Thuwal 23955\u20136900 Kingdom of Saudi Arabia"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Tianya","family":"Jin","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Polymer Physics and Chemistry, Changchun Institute of Applied Chemistry Chinese Academy of Sciences  Changchun 130022 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yang","family":"Liu","sequence":"additional","affiliation":[{"name":"College of Polymer Science and Engineering State Key Laboratory of Advanced Polymer Materials Sichuan University  Chengdu 610065 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zeng","family":"Chen","sequence":"additional","affiliation":[{"name":"Department of Chemistry Zhejiang University  Hangzhou 310027 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Dingqin","family":"Hu","sequence":"additional","affiliation":[{"name":"Chongqing Institute of Green and Intelligent Technology, Chongqing School, Chinese Academy of Sciences University of Chinese Academy of Sciences (UCAS Chongqing)  Chongqing 400714 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Wensu","family":"Long","sequence":"additional","affiliation":[{"name":"i\u2010Lab &amp; Printable Electronics Research Center, Suzhou Institute of Nano\u2010Tech and Nano\u2010Bionics Chinese Academy of Sciences (CAS)  Suzhou 215123 P. 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