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To satisfy various demands, state\u2010of\u2010the\u2010art OPSTs typically require multispectral responsiveness that is often pursued by leveraging the excellent optoelectronic properties and solution\u2010processability of quantum dots (QDs). However, this strategy suffers from complex fabrication procedures, limited mechanical flexibility and toxic cadmium\/lead compositions in QDs, which raise serious environmental and biosafety concerns. In this work, we demonstrate a fully solution\u2010processed and self\u2010supporting flexible OPST based on environmentally benign indium phosphide (InP) QDs. Through ligand exchange with fluorinated thiols, the QDs demonstrate improved photostability and enhanced energy level alignment with organic semiconductors. Furthermore, the interfacial dipole induced by fluorinated ligands enables long\u2010term charge retention. The resulting QD\u2010OPST devices exhibit broadband excitatory postsynaptic current (EPSC) responses, tunable synaptic plasticity, remarkable mechanical durability and ultralow energy consumption of 0.016 fJ, effectively mimicking cornea\u2010like nociceptor behaviors. In addition, the QD\u2010OPSTs display pronounced color selectivity, enabling blue\u2010feature recognition while suppressing red\u2010green background noise. This study provides a feasible strategy for developing high\u2010performance, eco\u2010friendly, and flexible photonic synapse devices, highlighting great potential for applications in visual perception and brain\u2010inspired computing.<\/jats:p>","DOI":"10.1002\/adma.202518057","type":"journal-article","created":{"date-parts":[[2025,12,27]],"date-time":"2025-12-27T09:59:45Z","timestamp":1766829585000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":10,"title":["Flexible Multiband Photonic Synapses for Nociceptive Perception and Neuromorphic Computation via Fluorinated InP Quantum Dots"],"prefix":"10.1002","volume":"38","author":[{"given":"Wanlong","family":"Lu","sequence":"first","affiliation":[{"name":"School of Physics and Optoelectronic Engineering Hangzhou Institute for Advanced Study University of Chinese Academy of Sciences  Hangzhou China"},{"name":"Research Center for Intelligent Manufacturing Computing Zhejiang Lab  Hangzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Peixian","family":"Li","sequence":"additional","affiliation":[{"name":"School of Physics and Optoelectronic Engineering Hangzhou Institute for Advanced Study University of Chinese Academy of Sciences  Hangzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Bin","family":"Zeng","sequence":"additional","affiliation":[{"name":"Research Center for Intelligent Manufacturing Computing Zhejiang Lab  Hangzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jing","family":"Wang","sequence":"additional","affiliation":[{"name":"Research Center for Intelligent Manufacturing Computing Zhejiang Lab  Hangzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ning","family":"Dai","sequence":"additional","affiliation":[{"name":"School of Physics and Optoelectronic Engineering Hangzhou Institute for Advanced Study University of Chinese Academy of Sciences  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