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Herein, to fully utilize active Pt sites to boost ethanol oxidation electrocatalysis, single\u2010Pt\u2010atoms anchored onto the surface of intermetallic Pd\n                    <jats:sub>5<\/jats:sub>\n                    Bi\n                    <jats:sub>3<\/jats:sub>\n                    core\u2010ultrathin Pd shell octahedrons, namely a tensile\u2010strained PdPt\n                    <jats:sub>1<\/jats:sub>\n                    SAA skin, were rationally designed and engineered. This unique PdPt\n                    <jats:sub>1<\/jats:sub>\n                    SAA skin achieves a record\u2010high mass activity (553.58 A mg\n                    <jats:sub>Pt<\/jats:sub>\n                    <jats:sup>\u22121<\/jats:sup>\n                    or 34.73 A mg\n                    <jats:sub>Pt+Pd<\/jats:sub>\n                    <jats:sup>\u22121<\/jats:sup>\n                    ) and outstanding durability toward ethanol oxidation in alkaline electrolyte, outperforming the current high\u2010performance electrocatalysts. Density functional theory (DFT) calculations reveal that the isolated\u2010Pt\u2010atoms effectively enhance the adsorption of ethanol, accelerate the C2 pathway, and enhance the C\u2010C bond cleavage of the *CH\n                    <jats:sub>2<\/jats:sub>\n                    CO intermediate. The wet\u2010chemical fabrication of SAA skin opens up a general strategy to construct model surface that completely exposes and stabilizes active atoms, facilitating the development of highly efficient electrocatalysts.\n                  <\/jats:p>","DOI":"10.1002\/adma.202519429","type":"journal-article","created":{"date-parts":[[2026,1,5]],"date-time":"2026-01-05T07:38:04Z","timestamp":1767598684000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":17,"title":["Maximize the Electrocatalytic Activity of Pt Toward Ethanol Oxidation via Engineering PdPt\n                    <sub>1<\/sub>\n                    Single\u2010Atom Alloy Skin"],"prefix":"10.1002","volume":"38","author":[{"ORCID":"https:\/\/orcid.org\/0009-0009-9767-2463","authenticated-orcid":false,"given":"Wen","family":"Chen","sequence":"first","affiliation":[{"name":"College of Civil and Transportation Engineering Shenzhen University  Shenzhen Guangdong P. R. China"},{"name":"Shenzhen Key Laboratory of Energy Electrocatalytic Materials Guangdong Provincial Key Laboratory of New Energy Materials Service Safety College of Materials Science and Engineering Shenzhen University  Shenzhen Guangdong P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Lei","family":"Xie","sequence":"additional","affiliation":[{"name":"Shenzhen Key Laboratory of Energy Electrocatalytic Materials Guangdong Provincial Key Laboratory of New Energy Materials Service Safety College of Materials Science and Engineering Shenzhen University  Shenzhen Guangdong P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yong","family":"Li","sequence":"additional","affiliation":[{"name":"Shenzhen Key Laboratory of Energy Electrocatalytic Materials Guangdong Provincial Key Laboratory of New Energy Materials Service Safety College of Materials Science and Engineering Shenzhen University  Shenzhen Guangdong P. R. 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China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Shao\u2010Qing","family":"Liu","sequence":"additional","affiliation":[{"name":"Shenzhen Key Laboratory of Energy Electrocatalytic Materials Guangdong Provincial Key Laboratory of New Energy Materials Service Safety College of Materials Science and Engineering Shenzhen University  Shenzhen Guangdong P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xian\u2010Zhu","family":"Fu","sequence":"additional","affiliation":[{"name":"Shenzhen Key Laboratory of Energy Electrocatalytic Materials Guangdong Provincial Key Laboratory of New Energy Materials Service Safety College of Materials Science and Engineering Shenzhen University  Shenzhen Guangdong P. R. 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