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One of the inherent bottlenecks lies on that the fullerenes would spontaneously aggregate into crystalline clusters at high temperature, causing the irreversible interface destruction. Herein, drawing inspiration from the bionic spider web, \u201cfullerene\u2010fixed web\u201d is constructed to firmly immobilize [6,6]\u2010phenyl\u2010C61\u2010butyric acid methyl ester (PCBM) molecules via in situ polymerized 3\u2010aminopropyltrimethoxysilane (APTMS)\u2010derived siloxane network. The hydrolyzed and polymerized APTMS forms a robust 3D framework that confines PCBM through strong hydrogen\u2010bonding interactions, thereby suppressing its thermal aggregation. Simultaneously, the exposed amino groups of the network passivate the perovskite surface defects and strengthen the perovskite\/ETL interfacial coupling. As a result, the target inverted PSCs achieve a champion efficiency of 26.39% (certified 26.27%) and retain over 90% of initial performance after 800 h age under ISOS\u2010L\u20103 condition\u2014significantly outperforming the control (24.98%, T\n                    <jats:sub>90<\/jats:sub>\n                    &lt; 250 h). This work provides a feasible and effective pathway toward achieving highly efficient and photothermally durable perovskite photovoltaics.\n                  <\/jats:p>","DOI":"10.1002\/adma.202520308","type":"journal-article","created":{"date-parts":[[2025,12,26]],"date-time":"2025-12-26T14:14:57Z","timestamp":1766758497000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":5,"title":["Suppressing Thermal Aggregation of Fullerene Enables ISOS\u2010L\u20103 Stable Inverted Perovskite Solar Cells"],"prefix":"10.1002","volume":"38","author":[{"given":"Qiang","family":"Weng","sequence":"first","affiliation":[{"name":"School of Physics and Electronic Science Engineering Research Center of Nano\u2010photonics and Advanced Instrument Ministry of Education East China Normal University  Shanghai 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