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Two\u2010dimensional (2D) nanomaterials with van der Waals layered structures have redefined the pursuit of superlubricity, where the interfacial potential corrugation is minimized by lattice incommensurability, and energy dissipation is further suppressed through phonon spectrum mismatch and charge\u2010mediated coupling at the sliding interface. These atomistic principles manifest in two archetypes of superlubricity: structural superlubricity, governed by interfacial misalignment that suppresses atomic registry, and transformation superlubricity, arising from shear\u2010induced interface reconstructions that dynamically smooth energy landscapes. Together they delineate a continuum from geometric misfit\u2010driven to shear\u2010adaptive energy dissipation modulation, yet translating these idealized states into device\u2010scale systems remains formidable, as scaling, environmental perturbations, and integration losses readily destabilize ultralow\u2010friction behavior. This review outlines how advances in van der Waals assembly, hybrid nanomembranes, and field\u2010tunable heterostructures have established three classes of sliding\u2010driven microsystems: mechanical energy transfer, mechano\u2010electrical conversion, and smart interfacial control. Looking ahead, the convergence of artificial intelligence (AI)\u2010guided design, standardized tribological metrics, and scalable integration is redefining superlubricity as a predictive framework for engineering 2D nanomaterials, nanoscale tribology, solid lubrication, superlubric interfaces, ultralow frictionreliable, energy\u2010efficient microdevices.<\/jats:p>","DOI":"10.1002\/adma.202520679","type":"journal-article","created":{"date-parts":[[2026,4,10]],"date-time":"2026-04-10T09:34:42Z","timestamp":1775813682000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":5,"title":["2D Nanomaterials Toward Function\u2010Ready Superlubricity in Advanced Microsystems"],"prefix":"10.1002","volume":"38","author":[{"given":"Yushan","family":"Geng","sequence":"first","affiliation":[{"name":"Department of Mechanical Engineering College of Engineering City University of Hong Kong  Kowloon Hong Kong SAR China"},{"name":"State Key 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