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However, the inherent chemical stability of CO\n                    <jats:sub>2<\/jats:sub>\n                    poses a grand challenge in achieving highly active and selective CO\n                    <jats:sub>2<\/jats:sub>\n                    conversion. Herein, we develop a biohybrid semi\u2010artificial photosynthetic system that integrates carbonic anhydrase (CA) and a CuZn nanozyme photosensitizer with a dendritic polymer (PPA) for the sustainable transformation of CO\n                    <jats:sub>2<\/jats:sub>\n                    into dimethyl carbonate (DMC). The PPA\u2010wrapped CA\/CuZn can capture CO\n                    <jats:sub>2<\/jats:sub>\n                    to form active intermediates. Through photo\u2010induced charge transfer under visible light illumination, the CA\/CuZn@PPA system achieves 100% selectivity for DMC production at room temperature and low CO\n                    <jats:sub>2<\/jats:sub>\n                    pressure.\n                  <\/jats:p>","DOI":"10.1002\/adma.202521092","type":"journal-article","created":{"date-parts":[[2025,12,19]],"date-time":"2025-12-19T10:08:12Z","timestamp":1766138892000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":1,"title":["Semi\u2010Artificial Photosynthetic Machinery for Carbon Dioxide Capture and Conversion"],"prefix":"10.1002","volume":"38","author":[{"given":"Shuting","family":"Huang","sequence":"first","affiliation":[{"name":"State Key Laboratory of Bioinspired Interfacial Materials Science, College of Chemistry Chemical Engineering and Materials Science Collaborative Innovation Center of Suzhou Nano Science and Technology Soochow University Suzhou P. 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