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Unfortunately, the construction of large\u2010sized and uniform integrated candidates with oriented microstructure remains an insurmountable challenge. Herein, we propose and demonstrate a novel large\u2010scale, highly uniform integrated oriented microstructured glass composite scintillator by triggering the oriented crystallization habit of the metastable glass. It is featured by columnar microcrystalline arrays with a high refractive index embedded in the glass phase with a relatively low refractive index. This enables to form an intrinsic waveguide configuration with light confinement capabilities, in which the directional propagation of photons can be realized. As a result, an excellent scintillation performance with the X\u2010ray excited luminescence intensity of 5.67 times that of BGO can be realized. It also demonstrates the excellent environmental resistance because of the all\u2010oxide system. By using this oriented microstructured glass composite scintillator, the X\u2010ray imaging system is built, and an impressive imaging resolution of 30 lp mm\n                    <jats:sup>\u22121<\/jats:sup>\n                    is successfully achieved. The progress represents a giant step toward high\u2010resolution X\u2010ray imaging with structured scintillators.\n                  <\/jats:p>","DOI":"10.1002\/adma.202521655","type":"journal-article","created":{"date-parts":[[2026,2,11]],"date-time":"2026-02-11T15:21:09Z","timestamp":1770823269000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":4,"title":["Oriented Microstructured Scintillator for High\u2010Resolution X\u2010Ray Imaging"],"prefix":"10.1002","volume":"38","author":[{"given":"Xunpiao","family":"Liu","sequence":"first","affiliation":[{"name":"State Key Laboratory of Luminescent Materials and Devices School of Materials Science and Engineering South China University of Technology  Guangzhou China"},{"name":"Guangdong Provincial Key Laboratory of Fiber Laser Materials and Applied Techniques Guangdong Engineering Technology Research Center of Special Optical Fiber Materials and Devices  Guangzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Dazhao","family":"Wang","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Luminescent Materials and Devices School of Materials Science and Engineering South China University of Technology  Guangzhou China"},{"name":"Guangdong Provincial Key Laboratory of Fiber Laser Materials and Applied Techniques Guangdong Engineering Technology Research Center of Special Optical Fiber Materials and Devices  Guangzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jianfeng","family":"Yan","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Luminescent Materials and Devices School of Materials Science and Engineering South China University of Technology  Guangzhou China"},{"name":"Guangdong Provincial Key Laboratory of Fiber Laser Materials and Applied Techniques Guangdong Engineering Technology Research Center of Special Optical Fiber Materials and Devices  Guangzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Shichao","family":"Lv","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Luminescent Materials and Devices School of Materials Science and Engineering South China University of Technology  Guangzhou China"},{"name":"Guangdong Provincial Key Laboratory of Fiber Laser Materials and Applied Techniques Guangdong Engineering Technology Research Center of Special Optical Fiber Materials and Devices  Guangzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ziang","family":"Liu","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Luminescent Materials and Devices School of Materials Science and Engineering South China University of Technology  Guangzhou China"},{"name":"Guangdong Provincial Key Laboratory of Fiber Laser Materials and Applied Techniques Guangdong Engineering Technology Research Center of Special Optical Fiber Materials and Devices  Guangzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Emmanuel","family":"Veron","sequence":"additional","affiliation":[{"name":"CNRS Univ. 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