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In situ fabrication of biocompatible electronics offers a promising strategy to achieve conformal skin\u2010electronic integration through intimate interfacial contact. However, existing in situ\u2010printable conductive inks face inherent trade\u2010offs between high conductivity and strong adhesion, as well as between environmental resilience and on\u2010demand removability, significantly limiting their practical utility. Here, we report a viscoelastic supramolecular polymer\u2010based conductive adhesive ink (AgBioA) that simultaneously achieves high electrical conductivity (&gt;15 000 S cm\n                    <jats:sup>\u22121<\/jats:sup>\n                    ), strong skin adhesion (\u223c3 N cm\n                    <jats:sup>\u22121<\/jats:sup>\n                    ), excellent environmental stability, ethanol\u2010triggered on\u2010demand dissolution, and superior biocompatibility. Our approach leverages a dynamically crosslinked supramolecular network, synthesized by copolymerizing \u03b1\u2010lipoic acid (LA) with 1,3\u2010diisopropenylbenzene (DIB) and reinforced with citric acid (CA) via hydrogen bonding. This unique design enables two key innovations: first, it ensures robust interfacial adhesion to diverse surfaces, from biological tissues to rigid electronic components; second, it facilitates the uniform dispersion of silver flakes into mechanically stable, percolated networks that guarantee highly reliable conductivity. Exploiting these advantages, we demonstrate fully integrated epidermal devices, including in situ fabricated bioelectrodes for reliable electrocardiography (ECG) and electrodermal activity (EDA) monitoring, and a skin\u2010conforming photoplethysmography (PPG) sensor where AgBioA functions dually as structural adhesive and conductive interconnect.\n                  <\/jats:p>","DOI":"10.1002\/adma.202521677","type":"journal-article","created":{"date-parts":[[2026,3,10]],"date-time":"2026-03-10T04:41:31Z","timestamp":1773117691000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":7,"title":["Highly Conductive Ag Flakes\u2010Based Bio\u2010Adhesive for Multi\u2010Functional Epidermal Electronics"],"prefix":"10.1002","volume":"38","author":[{"given":"Zujian","family":"Li","sequence":"first","affiliation":[{"name":"State Key Laboratory of Synergistic Chem\u2010Bio Synthesis, School of Chemistry and Chemical Engineering Zhangjiang Institute for Advanced Study National Center for Translational Medicine The International Peace Maternity and Child Health Hospital Shanghai Jiao Tong University  Shanghai P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Weichang","family":"Xie","sequence":"additional","affiliation":[{"name":"Department of Cardiovascular Surgery Ruijin Hospital Shanghai Jiao Tong University School of Medicine  Shanghai P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Tienan","family":"Zhao","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Synergistic Chem\u2010Bio Synthesis, School of Chemistry and Chemical Engineering Zhangjiang Institute for Advanced Study National Center for Translational Medicine The International Peace Maternity and Child Health Hospital Shanghai Jiao Tong University  Shanghai P. R. 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China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xiaofeng","family":"Ye","sequence":"additional","affiliation":[{"name":"Department of Cardiovascular Surgery Ruijin Hospital Shanghai Jiao Tong University School of Medicine  Shanghai P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Chunhai","family":"Fan","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Synergistic Chem\u2010Bio Synthesis School of Chemistry and Chemical Engineering Frontiers Science Center For Transformative Molecules National Center for Translational Medicine Institute of Molecular Medicine Shanghai Key Laboratory For Nucleic Acids Chemistry and Nanomedicine School of Medicine Renji Hospital Shanghai Jiao Tong University  Shanghai P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-1836-5609","authenticated-orcid":false,"given":"Zhitao","family":"Zhang","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Synergistic Chem\u2010Bio Synthesis, School of Chemistry and Chemical Engineering Zhangjiang Institute for Advanced Study National Center for Translational Medicine The International Peace Maternity and Child Health Hospital Shanghai Jiao Tong University  Shanghai P. R. China"},{"name":"Macao Translational Medicine Center Macau University of Science and Technology  Taipa Macau SAR P. R. 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