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Characterizing the elastic responses with atomic and femtosecond resolution across the magnetic transition is essential for guiding the design of magnetically tunable actuators and strain\u2010mediated spintronic devices. Here, ultrafast X\u2010ray diffraction employed at a free\u2010electron laser reveals that the atomic displacements, wave vectors, and dispersion relations of acoustic phonon modes in a vdW antiferromagnet FePS\n                    <jats:sub>3<\/jats:sub>\n                    are coupled with the magnetic order, by tracking both in\u2010plane and out\u2010of\u2010plane Bragg peaks upon optical excitation across the N\u00e9el temperature (\n                    <jats:italic>T<\/jats:italic>\n                    <jats:sub>N<\/jats:sub>\n                    ). One transverse mode shows that a quasi\u2010out\u2010of\u2010plane atomic displacement undergoes a significant directional change across\n                    <jats:italic>T<\/jats:italic>\n                    <jats:sub>N<\/jats:sub>\n                    . Its quasi\u2010in\u2010plane wave vector is derived by comparing the measured sound velocity and the first\u2010principles calculations. The other transverse mode is an interlayer shear acoustic mode whose amplitude is strongly enhanced in the antiferromagnetic phase, exhibiting eight times stronger amplitude than the longitudinal acoustic mode below\n                    <jats:italic>T<\/jats:italic>\n                    <jats:sub>N<\/jats:sub>\n                    . The atomically resolved characterization of acoustic phonon dynamics that couple with magnetic ordering opens opportunities for harnessing unique magnetoelastic coupling in vdW magnets on ultrafast timescales.\n                  <\/jats:p>","DOI":"10.1002\/adma.202522280","type":"journal-article","created":{"date-parts":[[2026,2,2]],"date-time":"2026-02-02T05:01:39Z","timestamp":1770008499000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":1,"title":["Atomically Resolved Acoustic Dynamics Coupled with Magnetic Order in a Van der Waals Antiferromagnet"],"prefix":"10.1002","volume":"38","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-8005-5620","authenticated-orcid":false,"given":"Faran","family":"Zhou","sequence":"first","affiliation":[{"name":"Materials Science Division Argonne National Laboratory  Lemont Illinois USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Kyle","family":"Hwangbo","sequence":"additional","affiliation":[{"name":"Department of Physics University of Washington  Seattle Washington USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Sung Soo","family":"Ha","sequence":"additional","affiliation":[{"name":"Center For Ultrafast Phase Transformation Department of Physics Sogang University  Seoul South Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xiao\u2010Wei","family":"Zhang","sequence":"additional","affiliation":[{"name":"Department of Materials Science and Engineering University of Washington  Seattle Washington USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Sae Hwan","family":"Chun","sequence":"additional","affiliation":[{"name":"Pohang Accelerator Laboratory POSTECH  Pohang Gyeongbuk South Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jaeku","family":"Park","sequence":"additional","affiliation":[{"name":"Pohang Accelerator Laboratory POSTECH  Pohang Gyeongbuk South Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Intae","family":"Eom","sequence":"additional","affiliation":[{"name":"Pohang Accelerator Laboratory POSTECH  Pohang Gyeongbuk South Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Qianni","family":"Jiang","sequence":"additional","affiliation":[{"name":"Department of Physics University of Washington  Seattle Washington USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zekai","family":"Yang","sequence":"additional","affiliation":[{"name":"Institute For Condensed Matter and Complex Systems School of Physics and Astronomy The University of Edinburgh  Edinburgh UK"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Marc","family":"Zajac","sequence":"additional","affiliation":[{"name":"Materials Science Division Argonne National Laboratory  Lemont Illinois USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Sungwon","family":"Kim","sequence":"additional","affiliation":[{"name":"Center For Ultrafast Phase Transformation Department of Physics Sogang University  Seoul South Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Sungwook","family":"Choi","sequence":"additional","affiliation":[{"name":"Center For Ultrafast Phase Transformation Department of Physics Sogang University  Seoul South Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-8285-7379","authenticated-orcid":false,"given":"Zhaodong","family":"Chu","sequence":"additional","affiliation":[{"name":"Materials Science Division Argonne National Laboratory  Lemont Illinois USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Kyoung Hun","family":"Oh","sequence":"additional","affiliation":[{"name":"Department of Physics Massachusetts Institute of Technology  Cambridge Massachusetts USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yifan","family":"Su","sequence":"additional","affiliation":[{"name":"Department of Physics Massachusetts Institute of Technology  Cambridge Massachusetts USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Alfred","family":"Zong","sequence":"additional","affiliation":[{"name":"Departments of Physics and Applied Physics Stanford University Stanford California USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Elton J. 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