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Here, we propose an electrostatic field attraction and in situ encapsulation synergistic strategy and demonstrate its effectiveness in an imine\u2010based adsorbent, IPIN\u2010P@MF. In this system, the polarized carboxylate groups in ionic polyimine network (IPIN) create a strong electrostatic field for directional iodine attraction, while multiple nitrogen sites and carbonyl\u2010rich additives enable chemical fixation through\n                    <jats:italic>N<\/jats:italic>\n                    \u2010methylation and complexation. This dual mechanism effectively addresses the limitations of conventional pore confinement approaches, allowing IPIN\u2010P@MF to achieve a record\u2010high dynamic I\n                    <jats:sub>2<\/jats:sub>\n                    uptake capacity of 160.7 wt.% at 150\u00b0C and 90% RH, and maintain filtration efficiency above 99.8% under simulated industrial conditions. The entire IPIN\u2010P@MF can be fabricated via solution processing under mild ambient conditions, offering remarkable cost\u2010effectiveness (0.126 USD per gram of iodine captured) and scalability (dimensions &gt;1.8 meters), thereby providing a practical and scalable pathway for radioactive iodine abatement in nuclear off\u2011gas treatment and emergency response.\n                  <\/jats:p>","DOI":"10.1002\/adma.202522566","type":"journal-article","created":{"date-parts":[[2026,4,11]],"date-time":"2026-04-11T07:21:58Z","timestamp":1775892118000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":1,"title":["Super Cost\u2010Effective and Scalable Imine\u2010Based Sorbent With Field Attraction and In Situ Fixation for Efficient Capture of Diverse Iodine Species under Industrial Conditions"],"prefix":"10.1002","volume":"38","author":[{"ORCID":"https:\/\/orcid.org\/0000-0001-9105-4247","authenticated-orcid":false,"given":"Guo\u2010Hao","family":"Zhang","sequence":"first","affiliation":[{"name":"CAEA Innovation Center of Nuclear Environmental Safety Technology College of Nuclear Science and Technology Southwest University of Science and Technology  Mianyang China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Wen\u2010Qi","family":"Zhang","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Radiation Medicine and Protection School of Radiation Medicine and Protection Collaborative Innovation Center of Radiological Medicine of Jiangsu Higher Education Institutions Soochow University  Suzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xue\u2010Yan","family":"Ren","sequence":"additional","affiliation":[{"name":"CAEA Innovation Center of Nuclear Environmental Safety Technology College of Nuclear Science 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and Technology Southwest University of Science and Technology  Mianyang China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Lin\u2010Ze","family":"Xiao","sequence":"additional","affiliation":[{"name":"CAEA Innovation Center of Nuclear Environmental Safety Technology College of Nuclear Science and Technology Southwest University of Science and Technology  Mianyang China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yun\u2010Long","family":"Zhang","sequence":"additional","affiliation":[{"name":"CAEA Innovation Center of Nuclear Environmental Safety Technology College of Nuclear Science and Technology Southwest University of Science and Technology  Mianyang China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Rui","family":"Li","sequence":"additional","affiliation":[{"name":"CAEA Innovation Center of Nuclear Environmental Safety Technology College of Nuclear Science and Technology Southwest University of Science and Technology  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