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Here, we report a heterogeneous\u2010network slippery liquid\u2010infused porous surface (SLIPS) coating engineered through a molecular design strategy. This design integrates a low\u2010surface\u2010energy rigid framework with a dynamic, self\u2010healing soft network. The rigid framework is formed by a cross\u2010linked network of thiol\u2010functionalized polyhedral oligomeric silsesquioxane (POSS\u2010(SH)\n                    <jats:sub>8<\/jats:sub>\n                    ) and fluorinated liquid nitrile rubber (F\n                    <jats:sub>13<\/jats:sub>\n                    \u2010LNBR). The soft network is based on a three\u2010arm cross\u2010linked structure constructed from hexamethylene\u2010diisocyanate isocyanurate trimer (THDI) and 2\u2010ureido\u20104[1H]\u2010pyrimidinone (UPy) units. Infused with silicone oil, the coating exhibits robust mechanical strength, demonstrated by an erosion rate of 74.37\u00a0nm\/s, and autonomous self\u2010healing capability enabled by multiple hydrogen bonds in both aerial and underwater conditions. Remarkably, the release rate of the silicone oil and the uniformity of surface hydrophobicity are precisely regulated by incorporating UPy units with tailored molecular structures and perfluoroacrylate monomers with varying hydrophobic chain lengths. Owing to these rational design elements, the coating repels a broad spectrum of fouling agents, including bacteria, algae, and highly viscous crude oil, while maintaining excellent flexibility and wear resistance. During a 90\u2010day field test in real seawater, the coating's transmittance decreased by only 5.8%. This synergistic design addresses key limitations in current SLIPS technologies, offering a viable pathway toward long\u2010term antifouling performance in challenging marine environments.\n                  <\/jats:p>","DOI":"10.1002\/adma.202522578","type":"journal-article","created":{"date-parts":[[2026,2,11]],"date-time":"2026-02-11T15:27:42Z","timestamp":1770823662000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":10,"title":["Heterogeneous Network SLIPS Coating with Soft\u2010Hard Chain Integration Design for Marine Antifouling Engineering"],"prefix":"10.1002","volume":"38","author":[{"ORCID":"https:\/\/orcid.org\/0009-0002-8951-9724","authenticated-orcid":false,"given":"Xuerui","family":"Zang","sequence":"first","affiliation":[{"name":"State Key Laboratory of Advanced Marine Materials Institute of Oceanology Chinese Academy of Sciences  Qingdao P. R. 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