{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,9,4]],"date-time":"2026-09-04T22:38:18Z","timestamp":1788561498655,"version":"build-2803163510"},"reference-count":33,"publisher":"Wiley","issue":"12","license":[{"start":{"date-parts":[[2026,1,21]],"date-time":"2026-01-21T00:00:00Z","timestamp":1768953600000},"content-version":"vor","delay-in-days":0,"URL":"http:\/\/onlinelibrary.wiley.com\/termsAndConditions#vor"},{"start":{"date-parts":[[2026,1,21]],"date-time":"2026-01-21T00:00:00Z","timestamp":1768953600000},"content-version":"tdm","delay-in-days":0,"URL":"http:\/\/doi.wiley.com\/10.1002\/tdm_license_1.1"}],"funder":[{"DOI":"10.13039\/501100012166","name":"National Key Research and Development Program of China","doi-asserted-by":"publisher","award":["2022YFB2402200"],"award-info":[{"award-number":["2022YFB2402200"]}],"id":[{"id":"10.13039\/501100012166","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["22479129"],"award-info":[{"award-number":["22479129"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["22350710185"],"award-info":[{"award-number":["22350710185"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":["advanced.onlinelibrary.wiley.com"],"crossmark-restriction":true},"short-container-title":["Advanced Materials"],"published-print":{"date-parts":[[2026,2]]},"abstract":"<jats:title>ABSTRACT<\/jats:title>\n                  <jats:p>\n                    The shuttle effect of lithium polyselenides (Li\n                    <jats:sub>2<\/jats:sub>\n                    Se\n                    <jats:sub>n<\/jats:sub>\n                    ) seriously hinders the practical application of lithium\u2212selenium (Li\u2212Se) batteries. Traditional approaches for confining Li\n                    <jats:sub>2<\/jats:sub>\n                    Se\n                    <jats:sub>n<\/jats:sub>\n                    cannot fundamentally resolve this issue. In this work, we adopt a strategy of in situ conversion of inorganic selenium into organic forms, which utilizes the nucleophilic reaction between Li\n                    <jats:sub>2<\/jats:sub>\n                    Se\n                    <jats:sub>n<\/jats:sub>\n                    and 2\u2212benzothiazole diethyldithiocarbamate (BTZA) to graft selenium atoms onto the organic framework. Upon charging, organic diselenides are generated, fundamentally eliminating the formation of Li\n                    <jats:sub>2<\/jats:sub>\n                    Se\n                    <jats:sub>n<\/jats:sub>\n                    . Furthermore, lithium benzothiazole sulfide (BTSLi) is concurrently produced during the organification process. It is converted to the redox\u2212active 2,2\u2032\u2212dibenzothiazole disulfide (BTDS) during charging, compensating for the capacity loss resulting from the C\u2212Se bond formation. Moreover, the organoselenium products exhibit high discharge voltages and strong lithium\u2212ion transport capability, enhancing the energy density and reaction kinetics of the battery. The Li\u2212Se cell with BTZA maintains a capacity retention of 92.87% after 1300 cycles at 2 C. The pouch cell with a capacity of 0.6 Ah can be stably operated for 30 cycles at 0.1 C. Excellent electrochemical performances are also achieved at high rates. This work presents a novel strategy for achieving highly stable Li\u2212Se battery.\n                  <\/jats:p>","DOI":"10.1002\/adma.202523054","type":"journal-article","created":{"date-parts":[[2026,1,21]],"date-time":"2026-01-21T09:27:56Z","timestamp":1768987676000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":3,"title":["In Situ Organoselenization for Ultrastable Li\u2212Se Batteries"],"prefix":"10.1002","volume":"38","author":[{"given":"Zhenggang","family":"Wang","sequence":"first","affiliation":[{"name":"College of Chemistry Zhengzhou University  Zhengzhou P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jiaxuan","family":"An","sequence":"additional","affiliation":[{"name":"College of Chemistry Zhengzhou University  Zhengzhou P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Kunchen","family":"Xie","sequence":"additional","affiliation":[{"name":"College of Chemistry Zhengzhou University  Zhengzhou P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zhuo","family":"Zhang","sequence":"additional","affiliation":[{"name":"College of Chemistry Zhengzhou University  Zhengzhou P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Qilong","family":"Yang","sequence":"additional","affiliation":[{"name":"College of Chemistry Zhengzhou University  Zhengzhou P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-3746-9884","authenticated-orcid":false,"given":"Yongzhu","family":"Fu","sequence":"additional","affiliation":[{"name":"College of Chemistry Zhengzhou University  Zhengzhou P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-7149-2802","authenticated-orcid":false,"given":"Wei","family":"Guo","sequence":"additional","affiliation":[{"name":"College of Chemistry Zhengzhou University  Zhengzhou P. R. 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