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Herein, we reveal that, under continuous high\u2010shear processing, the coupled effects of uncontrolled mechanical stress and frictional heating destroy mass\u2010transport channels and induce silent iodine loss. Inspired by low\u2010frequency mild mechanical actuation in respiratory systems, a targeted energy intermittent release strategy based on water\u2010cooled pulse shearing is proposed to achieve precise decoupling and regulation of mechanical force and frictional heat accumulation. It is revealed that maintaining energy input below the thresholds of carbon host structure damage and iodine desorption, avoids micro\u2010scale \u201cpore\u2010like\u201d structure exposed to the cracking of low\u2010crystallinity carbon, thereby preserving strong van der Waals confinement between carbon and iodine, fundamentally preventing abnormal iodine migration. Concurrently, regulating the energy within the window between PTFE fiber formation and fracture, contrasts a uniform and stable thick iodine electrode at the micro\u2010macro scale, which enables over 50000 stable cycles at 100 C and an ultra\u2010high area capacity of 16.27 mAh cm\n                    <jats:sup>\u22122<\/jats:sup>\n                    based on 82.84 mg\n                    <jats:sub>iodine<\/jats:sub>\n                    cm\n                    <jats:sup>\u22122<\/jats:sup>\n                    iodine loading. Importantly, a \u22481.2 Ah pouch cell even retains 98.5% capacity after 300 cycles at 2 C, demonstrating the scalability and practical viability of the strategy.\n                  <\/jats:p>","DOI":"10.1002\/adma.73037","type":"journal-article","created":{"date-parts":[[2026,4,11]],"date-time":"2026-04-11T17:25:41Z","timestamp":1775928341000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":23,"title":["Mechanical\u2010Thermal Decoupling Engineering Unlocks Ultra\u2010Stable Dry Thick Iodine Cathodes for Ah\u2010Level Zinc\u2010Based Pouch Batteries"],"prefix":"10.1002","volume":"38","author":[{"given":"Hengrui","family":"Guo","sequence":"first","affiliation":[{"name":"School of Materials Science and Engineering Xiamen University of Technology  Xiamen Fujian China"},{"name":"School of Materials Science and Engineering Zhengzhou University  Zhengzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Hao","family":"Luo","sequence":"additional","affiliation":[{"name":"School of Materials Science and Engineering Xiamen University of Technology  Xiamen Fujian China"},{"name":"School of Materials Science and Engineering Zhengzhou University  Zhengzhou China"},{"name":"Laboratory of Advanced Materials Aqueous Battery Center College of Smart Materials and Future Energy Fudan University  Shanghai P. 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