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Herein, we have first proposed a synergistic strategy by patterned blade\u2010coating with modulation of multicomponent fragmental entropy effect to construct pseudo\u2010planar heterojunction (PPHJ) all\u2010PSCs with an ideal vertical gradient distribution. The patterned blades allow polymer fluid to be extruded in a confined space, which can enhance the directional shear capability during the printing process, thus effectively guiding the stretching of polymer chains. Furthermore, the introduction of PTQ10 with favorable packing orientation can effectively bind with PM6 fragments to suppress the entropy\u2010driven retraction effect and alleviate excessive aggregation of PM6 fragments, which is beneficial to form PPHJ structure with favorable phase separation. Therefore, the device based on PM6:PTQ10\/PY\u2010DT system exhibits a competitive power conversion efficiency (PCE) of 19.78%, with a fill factor of nearly 80%. Notably, the corresponding 16.94 cm\n                    <jats:sup>2<\/jats:sup>\n                    flexible module achieves PCE of 16.08%. These results indicate directional fluid force guidance and ordered polymer fragments stacking are key for dual\u2010fiber morphology, providing a reliable approach for all\u2010PSCs commercialization.\n                  <\/jats:p>","DOI":"10.1002\/adma.73084","type":"journal-article","created":{"date-parts":[[2026,4,17]],"date-time":"2026-04-17T10:31:46Z","timestamp":1776421906000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Pattern\u2010Induced Directional Shear Force Synergized With Regulation of Multicomponent Fragments Entropy Effect for Printable Efficiency All\u2010Polymer Solar Cells"],"prefix":"10.1002","volume":"38","author":[{"given":"Zetong","family":"Wang","sequence":"first","affiliation":[{"name":"College of Chemistry and Chemical Engineering\/Film Energy Chemistry for Jiangxi Provincial Key Laboratory (FEC)\/Institute of Polymers and Energy Chemistry (IPEC) Nanchang University  Nanchang 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