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A clear understanding of spin effects and effective strategies for spin regulation is therefore essential for advancing CO\n                    <jats:sub>2<\/jats:sub>\n                    conversion catalysis. This review briefly summarizes recent advances in the underlying mechanisms and a few representative examples of spin\u2010enhanced CO\n                    <jats:sub>2<\/jats:sub>\n                    conversion, highlighting their importance in steering CO\n                    <jats:sub>2<\/jats:sub>\n                    conversion toward high value\u2010added products. It begins with an introduction to spin\u2010dependent reaction pathways and spin regulation at catalytic active sites, followed by a discussion of emerging approaches for spin\u2010enhanced CO\n                    <jats:sub>2<\/jats:sub>\n                    conversion. Spin catalysis strategies based on external magnetic fields and internal magnetic interactions are presented, highlighting their roles in promoting photocatalytic and electrocatalytic CO\n                    <jats:sub>2<\/jats:sub>\n                    reduction toward diverse and value\u2010added products. Besides,\n                    <jats:italic>in situ\/operando<\/jats:italic>\n                    characterization techniques are essential for exploring the underlying mechanisms of spin catalysis and tracking the spin\u2010sensitive reaction intermediates during CO\n                    <jats:sub>2<\/jats:sub>\n                    conversion. Finally, key challenges and future opportunities in the design of spin catalysts, as well as the reactor engineering for practical applications, are discussed, advancing the concept of spin catalysis for achieving sustainable CO\n                    <jats:sub>2<\/jats:sub>\n                    conversion.\n                  <\/jats:p>","DOI":"10.1002\/adma.73300","type":"journal-article","created":{"date-parts":[[2026,5,9]],"date-time":"2026-05-09T06:03:42Z","timestamp":1778306622000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":3,"title":["The Emergence of Spin\u2010Enhanced Catalysis for CO\n                    <sub>2<\/sub>\n                    Conversion"],"prefix":"10.1002","volume":"38","author":[{"given":"Bojun","family":"Shi","sequence":"first","affiliation":[{"name":"Key Laboratory of Photochemistry Beijing National Laboratory For Molecular Sciences Institute of Chemistry Chinese Academy of Sciences  Beijing 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