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However, due to the limited research on pseudocapacitive film electrode materials, achieving high energy density for film supercapacitor remains a challenge. Here, the film anode (Fe@Fe\n                    <jats:sub>3<\/jats:sub>\n                    O\n                    <jats:sub>4<\/jats:sub>\n                    \/CNTs) and cathode (NiCo\u2010NiCo compound\/CNTs) were prepared by the vacuum filtration technology. Density functional theory calculations combined with experimental results revealed that oxygen vacancies can induce the formation of dense localized charge aggregation regions at the Fe\/Fe\n                    <jats:sub>3<\/jats:sub>\n                    O\n                    <jats:sub>4<\/jats:sub>\n                    interface, significantly enhancing the charge transfer rate in electrochemical reactions, enabling the anode to achieve a specific capacity of 7.88 F cm\n                    <jats:sup>\u22122<\/jats:sup>\n                    (749.1 C g\n                    <jats:sup>\u22121<\/jats:sup>\n                    ) at a high mass loading of 16.7\u00a0mg cm\n                    <jats:sup>\u22122<\/jats:sup>\n                    . Meanwhile, after introducing oxygen vacancies, the adhesion energy at the interface significantly increased, enhancing the binding strength between Fe and Fe\n                    <jats:sub>3<\/jats:sub>\n                    O\n                    <jats:sub>4<\/jats:sub>\n                    , making it less prone to peeling due to current shock during long\u2010term charge and discharge cycles, thereby improving the cycling stability of the Fe\u2010based anode (76% capacitance retention after 20\u00a0000 cycles). The all\u2010pseudocapacitive film supercapacitor successfully assembled obtains an excellent energy density of 1.362 mWh cm\n                    <jats:sup>\u22122<\/jats:sup>\n                    (122.5\u00a0Wh kg\n                    <jats:sup>\u22121<\/jats:sup>\n                    ) at a total mass loading of 27.8\u00a0mg cm\n                    <jats:sup>\u22122<\/jats:sup>\n                    , far exceeding previously reported values.\n                  <\/jats:p>","DOI":"10.1002\/adma.73302","type":"journal-article","created":{"date-parts":[[2026,5,6]],"date-time":"2026-05-06T13:20:17Z","timestamp":1778073617000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":3,"title":["Magnetically Induced Ordered Structure\u2010Assisted Defect Engineering Strategy for High\u2010Performance All\u2010Pseudocapacitive Film 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