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In this work, a distinctive supramolecular\/polymer conjoined\u2010network is proposed to overcome the long\u2010standing stiffness\u2010energy dissipation dilemma. By exchanging from a good solvent to a poor one, the intra\u2010 and intermolecular noncovalent interactions between supramolecular gelators and polymers are initially suppressed and then recovered, generating a supramolecular network and a polymer network, noncovalently conjoined with each other. This conjoined\u2010network structure is found to deform affinely, preventing unexpected stress concentration, thus yielding favorable combined mechanical properties. When deformed, those supramolecular and polymer domains initially survive to arrest deformation, while later adaptively disassemble and fracture to dissipate substantial energy through diverse pathways and across multiple scales, enabling the desirable compatibility between stiffness and energy dissipation. Consequently, the supramolecular\/polymer conjoined\u2010network hydrogel achieves coordinatively enhanced stiffness (10\u201332 MPa) and energy dissipation (dissipated energy of 6\u201312 MJ\/m\n                    <jats:sup>3<\/jats:sup>\n                    and dissipation coefficient up to 99%), collectively providing superior impact resistance and shock attenuation to extend their application as structural materials.\n                  <\/jats:p>","DOI":"10.1002\/adma.73369","type":"journal-article","created":{"date-parts":[[2026,5,14]],"date-time":"2026-05-14T06:15:41Z","timestamp":1778739341000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":2,"title":["Supramolecular Interaction Mediated Affine Deformation for Energy\u2010Dissipative Stiff Hydrogel"],"prefix":"10.1002","volume":"38","author":[{"given":"Liju","family":"Xu","sequence":"first","affiliation":[{"name":"Beijing National Laboratory for Molecular Sciences Laboratory of Polymer Physics and Chemistry CAS Research\/Education Center for Excellence in Molecular Sciences Institute of Chemistry Chinese Academy of Sciences  Beijing China"},{"name":"School of Chemical Sciences University of Chinese Academy of Sciences  Beijing China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Baokui","family":"Li","sequence":"additional","affiliation":[{"name":"Beijing National Laboratory for Molecular Sciences Laboratory of Polymer Physics and Chemistry CAS Research\/Education Center for Excellence in Molecular Sciences Institute of Chemistry Chinese Academy of Sciences  Beijing China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Bolin","family":"Wan","sequence":"additional","affiliation":[{"name":"Beijing National Laboratory for Molecular Sciences Laboratory of Polymer Physics and Chemistry CAS Research\/Education Center for Excellence in Molecular Sciences Institute of Chemistry Chinese Academy of Sciences  Beijing 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