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However, achieving integrated high stretchability, stable electrical performance, and long\u2010term durability in protein\u2010based sensing materials remains a critical challenge. Conventional modification strategies are largely confined to molecular\u2010scale adjustments, which often fail to simultaneously address these functional demands. This study introduces a fundamentally different approach by leveraging Hofmeister\u2010ion engineering to directly regulate the aggregation structure of tropocollagen, which enables a structural transformation from long\u2010range order to entropy\u2010driven disorder. Unlike previous methods that rely on chemical crosslinking or exogenous additives, our strategy selectively disrupts collagen's supramolecular order while preserving its triple\u2010helical integrity, resulting in a highly stretchable and conductive ionic gel with exceptional elasticity (fracture strain 560.00%, elastic range 300.53%, resilience 97.36%), durable ionic conductivity (0.56\u00a0S\u00a0m\n                    <jats:sup>\u22121<\/jats:sup>\n                    ), and reliable sensing performance over 1500 tensile cycles. By establishing a new paradigm of mesoscale disordering, this work not only deepens the understanding of ion\u2010modulated hierarchical assembly but also provides a versatile, biocompatible platform for next\u2010generation flexible electronics, soft robotics, and implantable sensing systems.\n                  <\/jats:p>","DOI":"10.1002\/adma.73545","type":"journal-article","created":{"date-parts":[[2026,6,2]],"date-time":"2026-06-02T14:55:28Z","timestamp":1780412128000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":4,"title":["Ordered\u2013Disorder Transition Induced Stretchable Collagen Ionic Gels Toward Flexible Sensors"],"prefix":"10.1002","volume":"38","author":[{"ORCID":"https:\/\/orcid.org\/0000-0001-9631-3738","authenticated-orcid":false,"given":"Ying","family":"Pei","sequence":"first","affiliation":[{"name":"College of Materials Science and Engineering Zhengzhou University  Zhengzhou 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