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Notably, metal halide perovskites with superior optoelectronic properties show great prospects for optical sensing technology. However, the current processing techniques of perovskite materials are mainly solution methods and vapor\u2010phase methods, facing toxic solvents and material waste, which are harmful to the natural environment and human health. Herein, we originally developed the temperature field\u2010driven directional space\u2010confined melt crystallization strategy, which perfectly solved the problems of toxic solvent and material waste, yielding highly crystalline, purely oriented 2D perovskite single\u2010crystal films. Long\u2010range\u2010oriented single\u2010crystal films with fewer crystal domains and defects ensure that optical synaptic devices possess image encryption and high\u2010fidelity polarization imaging capabilities. Furthermore, the melt processing technique enables the fabrication of high\u2010quality 2D\u20103D perovskite heterojunctions, which notably improve the photodetector performance of 2D perovskite. This pioneering work provides a new strategy and opportunity for the environmentally friendly, high\u2010throughput integration of perovskite optoelectronic devices.<\/jats:p>","DOI":"10.1002\/adma.73597","type":"journal-article","created":{"date-parts":[[2026,6,2]],"date-time":"2026-06-02T11:05:33Z","timestamp":1780398333000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Temperature Field\u2010Driven Directional Space\u2010Confined Crystallization of Perovskite Melt Toward High\u2010Performance Optoelectronic Devices"],"prefix":"10.1002","volume":"38","author":[{"given":"Yi","family":"Hao","sequence":"first","affiliation":[{"name":"College of Chemistry and Pingyuan Laboratory Zhengzhou University  Zhengzhou P. R. 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