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Herein, we report a SAM regulation strategy by mixing hydroxylated V\n                    <jats:sub>2<\/jats:sub>\n                    CT\n                    <jats:sub>x<\/jats:sub>\n                    MXene (V\n                    <jats:sub>2<\/jats:sub>\n                    C\u2010OH) with nickel oxide (NiO\n                    <jats:sub>x<\/jats:sub>\n                    ), which can provide abundant hydroxyl sites for SAM anchoring, thereby forming a uniform and dense SAM layer. First\u2010principles calculations further reveal that the binding energy between SAM and hydroxyl groups on V\n                    <jats:sub>2<\/jats:sub>\n                    C\u2010OH is stronger than that on pristine NiO\n                    <jats:sub>x<\/jats:sub>\n                    , explaining the enhanced thermal stability of SAM on the hybrid substrate. Meanwhile, the highly ordered and tightly packed SAM layer promotes vertical growth and [001]\u2010preferred orientation of perovskite grains. Therefore, the introduction of V\n                    <jats:sub>2<\/jats:sub>\n                    C\u2010OH enables a top\u2010down modulation of the NiO\n                    <jats:sub>x<\/jats:sub>\n                    , SAM, and perovskite layers, improving their morphology and interfacial properties. The resulting PSCs achieve a champion power conversion efficiency of 26.6% (certified at 26.2%) for a 0.0524 cm\n                    <jats:sup>2<\/jats:sup>\n                    device and 24.7% for a 1 cm\n                    <jats:sup>2<\/jats:sup>\n                    device, along with outstanding long\u2010term operational stability.\n                  <\/jats:p>","DOI":"10.1002\/adma.73656","type":"journal-article","created":{"date-parts":[[2026,6,8]],"date-time":"2026-06-08T07:00:12Z","timestamp":1780902012000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":3,"title":["Hydroxyl Interfacial Engineering for Self\u2010Assemble Monolayers Anchoring on NiO\n                    <sub>x<\/sub>\n                    Enables Efficient and Stable Perovskite Solar Cells"],"prefix":"10.1002","volume":"38","author":[{"given":"Xianzhao","family":"Wang","sequence":"first","affiliation":[{"name":"Key Laboratory of Physics and Technology for Advanced Batteries (Ministry of Education) College of Physics Jilin University  Changchun China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Qingyuan","family":"Zhao","sequence":"additional","affiliation":[{"name":"Key Laboratory of Physics and Technology for Advanced Batteries (Ministry of Education) College of Physics Jilin University  Changchun China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Lin","family":"Yang","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Integrated Optoelectronics Key Laboratory for UV\u2010Emitting Materials and Technology of Ministry of Education Northeast Normal University  Changchun China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ziyan","family":"Liu","sequence":"additional","affiliation":[{"name":"Graduate School of Engineering Toin University of Yokohama  Yokohama Kanagawa Japan"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yanxiang","family":"Liu","sequence":"additional","affiliation":[{"name":"School of Physics and Advanced Energy Henan University of Technology  Zhengzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Chunhui","family":"Geng","sequence":"additional","affiliation":[{"name":"Key Laboratory of Physics and Technology for Advanced Batteries (Ministry of Education) College of Physics Jilin University  Changchun China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Tianfang","family":"Zheng","sequence":"additional","affiliation":[{"name":"Key Laboratory of Physics and Technology for Advanced Batteries (Ministry of Education) College of Physics Jilin University  Changchun China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yisong","family":"Zheng","sequence":"additional","affiliation":[{"name":"Key Laboratory of Physics and Technology for Advanced Batteries (Ministry of Education) College of Physics Jilin University  Changchun China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Aijun","family":"Li","sequence":"additional","affiliation":[{"name":"Key Laboratory of Physics and Technology for Advanced Batteries (Ministry of Education) College of Physics Jilin University  Changchun China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-2182-049X","authenticated-orcid":false,"given":"Naoyuki","family":"Shibayama","sequence":"additional","affiliation":[{"name":"Graduate School of Engineering Toin University of Yokohama  Yokohama Kanagawa Japan"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Tsutomu","family":"Miyasaka","sequence":"additional","affiliation":[{"name":"Graduate School of Engineering Toin University of Yokohama  Yokohama Kanagawa 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