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Here, we report molecular spintronic devices featuring vertically asymmetric nanocolumn channels formed by phase separation. These channels confine spins and generate built\u2010in electric fields, boosting room\u2010temperature\n                    <jats:italic>\u03b7<\/jats:italic>\n                    <jats:sub>s<\/jats:sub>\n                    to 20%\u2014the highest value reported to date, over five times that of unstructured films. Simultaneously, the nanocolumn channels induce pronounced bias\u2010dependent asymmetry, with\n                    <jats:italic>\u03b7<\/jats:italic>\n                    <jats:sub>s<\/jats:sub>\n                    of 20% at +0.2\u00a0V versus 1% at \u22120.2\u00a0V, yielding a record asymmetry factor, significantly outperforming other material systems (e.g., metal oxides, 2D materials, conventional molecular\/inorganic semiconductors). This dual achievement of record\u2010high efficiency and strong asymmetry establishes a platform for new spintronic functionalities. As a proof of concept, we demonstrate its potential for information\u2010secure applications via spin\u2010signal encryption elements and two\u2010stage spin true random number generators, integrating structural design with spintronic operation.\n                  <\/jats:p>","DOI":"10.1002\/adma.73826","type":"journal-article","created":{"date-parts":[[2026,6,29]],"date-time":"2026-06-29T15:45:23Z","timestamp":1782747923000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["High\u2010Efficiency Asymmetric Spin Transport Enabled by Nanocolumn Molecular Semiconductors"],"prefix":"10.1002","volume":"38","author":[{"given":"Shunhua","family":"Hu","sequence":"first","affiliation":[{"name":"Laboratory of Nanosystem and Hierarchical Fabrication, Laboratory of Theoretical and Computational Nanoscience, Laboratory of Standardization and Measurement for Nanotechnology National Center for Nanoscience and Technology  Beijing P. 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