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Unlike traditional pigment\u2010based colors, which can fade, structural colored pigments are generated by intricate microscopic structures that manipulate light, resulting in intense iridescence and metallic sheens. The development of structural colored pigments presents a critical opportunity to replace traditional toxic colorants with safe, sustainable alternatives. Inspired from the nature, self\u2010assembly of different polymeric building blocks including colloidal nanoparticles, cellulose nanocrystals, and block copolymers, have been reported to fabricate photonic pigment. This review focuses on the summary of various polymeric building blocks, preparation strategies, and optical properties. Meanwhile, the state\u2010of\u2010the\u2010art applications are discussed, including macroscopic photonic materials, colorimetric sensors, painting and drug delivery. 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