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Continuous large\u2010scale fabrication of this crosslinked system is realized using a unique channel\u2010confinement strategy. By innovatively designing the end\u2010group molecular structures of linear polymers, we precisely regulate the liquid\u2010crystal phases within the semi\u2010interpenetrating network fibers. Four distinct liquid\u2010crystal phases are constructed, mimicking the \u03b2\u2010sheet nanocrystals of spider silk to enable efficient energy dissipation. The resulting fibers exhibit a high elastic modulus of 47.6\u00a0MPa, outstanding toughness of 60.4\u00a0MJ m\n                    <jats:sup>\u22123<\/jats:sup>\n                    , a high dissipation coefficient of 88.6%, an ultra\u2010broad damping temperature window, a wide damping frequency range, and a strong actuation stress. When woven into damping nets for impact buffering, the nets exhibit a tunable memory recovery time and an exceptionally low dynamic rebound ratio of 5.9%, enabling efficient impact\u2010energy adsorption and secure capture. Overall, this work overcomes the long\u2010standing trade\u2010off among mechanical, actuation performance, and damping capacity of LCEs, and provides a universal strategy for elastomer\u2010based damper design and precise liquid crystal phase control, opening new opportunities for applications in elastomer dampers, artificial muscles, and soft robotic systems.\n                  <\/jats:p>","DOI":"10.1002\/adma.73958","type":"journal-article","created":{"date-parts":[[2026,7,9]],"date-time":"2026-07-09T07:18:27Z","timestamp":1783581507000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":1,"title":["Spider Silk\u2010Inspired High\u2010Damping Liquid Crystal Elastomer Fibers Enabled by Semi\u2010Interpenetrating Networks"],"prefix":"10.1002","volume":"38","author":[{"given":"Xiao","family":"Liu","sequence":"first","affiliation":[{"name":"State Key Laboratory of Medicinal Chemical Biology Frontiers Science Center for New Organic Matter Key Laboratory of Functional Polymer Materials Tianjin Key Laboratory of Functional Polymer Materials College of Chemistry Nankai University  Tianjin China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Li","family":"Song","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Medicinal Chemical Biology Frontiers Science Center for New Organic Matter Key Laboratory of Functional Polymer Materials Tianjin Key Laboratory of Functional Polymer Materials College of Chemistry Nankai University  Tianjin China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Wang","family":"Chang","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Medicinal Chemical Biology Frontiers Science Center for New Organic Matter Key Laboratory of Functional Polymer Materials Tianjin Key Laboratory of Functional Polymer Materials College of Chemistry Nankai University  Tianjin China"},{"name":"Center of Drug Discovery, State Key Laboratory of Natural Medicines, Department of Science, School of Traditional Chinese Pharmacy China Pharmaceutical University Nanjing China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Shaoli","family":"Fang","sequence":"additional","affiliation":[{"name":"Alan G. 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