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It remains highly desirable to convert agricultural residues into high\u2010performance regenerated cellulose fibers in a green and scalable manner. However, the fabrication of superior agricultural regenerated fibers is demanding due to the inherent anti\u2010depolymerization structure and low degree of polymerization of agricultural cellulose. Here, we demonstrated a recyclable and eco\u2010efficient process enabling the selective extraction of cellulose from agricultural residues using a novel acid deep eutectic solvent system, and proposed a stretch\u2010induced alignment and spatial confinement strategy to realize scalable fabrication of high\u2010strength and high\u2010toughness regenerated fibers. The deep eutectic solvent presented efficient delignification and tailoring capacity for agricultural residue, yielding cellulose with a high purity of 91.2% and a crystallinity of 72.6%. The resultant fibers addressed the intrinsic limitations of agricultural cellulose through the formation of aligned nanofibril structures and densified hydrogen\u2010bonding networks, exhibiting a tensile strength of 852\u00a0MPa and a toughness of 110\u00a0MJ m\n                    <jats:sup>\u22123<\/jats:sup>\n                    . This work establishes a foundational pathway for producing high\u2010performance bio\u2010based fibers derived from agricultural residues, advancing sustainable materials innovation and circular bioeconomy development.\n                  <\/jats:p>","DOI":"10.1002\/adma.74131","type":"journal-article","created":{"date-parts":[[2026,7,18]],"date-time":"2026-07-18T12:11:27Z","timestamp":1784376687000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":1,"title":["An Eco\u2010Efficient and Sustainable Strategy for Fabricating High\u2010Strength Agricultural Fibers"],"prefix":"10.1002","volume":"38","author":[{"given":"Qi","family":"Tang","sequence":"first","affiliation":[{"name":"Shanghai Frontiers Science Center of Advanced Textiles College of Textiles Donghua University  Shanghai China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Mingjuan","family":"Du","sequence":"additional","affiliation":[{"name":"Shanghai 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