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Here, an angstrom\u2013scale confined ion sieve and accelerator is designed using unilamellar Ti\n                    <jats:sub>0.87<\/jats:sub>\n                    O\n                    <jats:sub>2<\/jats:sub>\n                    nanosheets with atomic Ti vacancies (\u223c3.0 \u00d7 3.8 \u00c5) and interlayer spacing (\u223c3.5 \u00c5) to enable selective Zn\n                    <jats:sup>2+<\/jats:sup>\n                    (\u223c1.5 \u00c5) transport while blocking H\n                    <jats:sub>2<\/jats:sub>\n                    O (\u223c4.0 \u00c5) and SO\n                    <jats:sub>4<\/jats:sub>\n                    <jats:sup>2\u2212<\/jats:sup>\n                    (\u223c5.9 \u00c5). This design facilitates selective Zn\n                    <jats:sup>2+<\/jats:sup>\n                    ion transport with high flux and Zn\/SO\n                    <jats:sub>4<\/jats:sub>\n                    <jats:sup>2\u2212<\/jats:sup>\n                    selectivity, effectively mitigating water\u2013\/anion\u2013induced parasitic reactions at the Zn anode. Consequently, the Ti\n                    <jats:sub>0.87<\/jats:sub>\n                    O\n                    <jats:sub>2<\/jats:sub>\n                    @Zn anode exhibits significantly suppressed dendrite growth and parasitic side reactions during repeated Zn plating\/stripping, with stable cycle lives exceeding 5000 and 4000 h at 1 and 5\u00a0mA cm\n                    <jats:sup>\u22122<\/jats:sup>\n                    , respectively. The Ah\u2013level Ti\n                    <jats:sub>0.87<\/jats:sub>\n                    O\n                    <jats:sub>2<\/jats:sub>\n                    @Zn\/\/VO\n                    <jats:sub>2<\/jats:sub>\n                    pouch cell retains 85.4% of its initial capacity after 300 cycles at 3 A g\n                    <jats:sup>\u22121<\/jats:sup>\n                    . This strategy provides a promising interfacial design concept for improving the reversibility of aqueous Zn metal anodes and may inspire the rational design of confined ion\u2013transport interphases for related aqueous battery systems.\n                  <\/jats:p>","DOI":"10.1002\/adma.74289","type":"journal-article","created":{"date-parts":[[2026,7,29]],"date-time":"2026-07-29T07:32:47Z","timestamp":1785310367000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":1,"title":["Angstrom\u2010Scale Confined Ion Sieve and Accelerator for Efficient Aqueous Zinc Batteries"],"prefix":"10.1002","volume":"38","author":[{"given":"Xing","family":"Peng","sequence":"first","affiliation":[{"name":"School of Chemistry and Chemical Engineering Key Laboratory for Soft Chemistry and Functional Materials of Ministry of Education Nanjing University of Science and Technology  Nanjing 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