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Here, a highly crystallized Cr\n                    <jats:sup>3+<\/jats:sup>\n                    \u2010doped transparent glass composite is reported that breaks this conventional compromise, delivering an optical transmittance exceeding 80% and a near\u2010unity internal quantum efficiency of 98.5%. Under x\u2010ray excitation, the glass composite exhibits a radioluminescence (RL)\u00a0intensity five times that of Bi\n                    <jats:sub>4<\/jats:sub>\n                    Ge\n                    <jats:sub>3<\/jats:sub>\n                    O\n                    <jats:sub>12<\/jats:sub>\n                    and shows thermally enhanced RL, reaching 105% of its room\u2010temperature intensity at 150\u00b0C. This functionality is further extended to fiber form, where NIR glass composite fibers are realized. High\u2010resolution x\u2010ray imaging is achieved with a spatial resolution of 27 lp mm\n                    <jats:sup>\u22121<\/jats:sup>\n                    , while integration of optical and x\u2010ray excitation pathways further enables cooperative dual\u2010modal imaging with complementary contrast and enhanced information depth. These results demonstrate a viable strategy for integrating optical transparency, NIR emission and x\u2010ray response within a single material platform, supporting advanced photonic and imaging applications.\n                  <\/jats:p>","DOI":"10.1002\/adma.74454","type":"journal-article","created":{"date-parts":[[2026,8,5]],"date-time":"2026-08-05T10:48:39Z","timestamp":1785926919000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Highly Crystallized Transparent Composite for Cooperative Imaging"],"prefix":"10.1002","volume":"38","author":[{"ORCID":"https:\/\/orcid.org\/0000-0003-3005-9145","authenticated-orcid":false,"given":"Quan","family":"Dong","sequence":"first","affiliation":[{"name":"State Key Laboratory of Luminescent Materials and Devices School of Materials Science and Engineering Guangdong Engineering Technology Research and Development Center of Special Optical Fiber Materials and Devices Guangdong Provincial Key Laboratory of Fiber Laser Materials and Applied Techniques South China University of Technology  Guangzhou P. R. China"},{"name":"Key Laboratory of Testing and Tracing of Rare Earth Products State Administration for Market Regulation Jiangxi University of Science and Technology  Ganzhou P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Dazhao","family":"Wang","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Luminescent Materials and Devices School of Materials Science and Engineering Guangdong Engineering Technology Research and Development Center of Special Optical Fiber Materials and Devices Guangdong Provincial Key Laboratory of Fiber Laser Materials and Applied Techniques South China University of Technology  Guangzhou P. R. 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