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Inspired by the gating mechanism of biological transient receptor potential (TRP) ion channels, we propose a hydrogen\u2010bond trap regulation strategy. By constructing localized hydrogen\u2010bond traps with heterogeneous energy distributions within a deep eutectic solvent (DES) gel network, continuous ion transport is transformed into a confined, thermally activated hopping process. This approach yields an ultrahigh temperature coefficient of resistance (TCR) of 178% \u00b0C\n                    <jats:sup>\u22121<\/jats:sup>\n                    and a high\n                    <jats:italic>B<\/jats:italic>\n                    value of 7880 K. A miniature flexible probe (\u00d81.0\u00a0mm \u00d7 1.0\u00a0mm) demonstrates practical potential in organ temperature monitoring and wireless respiratory tracking. The tailored hydrogen\u2010bond traps also effectively suppress multimodal crosstalk, enabling the fabrication of a decoupled trimodal sensing system that independently resolves proximity, pressure, and temperature signals for human\u2013robot interaction. This work establishes a versatile materials strategy for achieving thermal perception in soft electronics and provides a general platform for tuning ion transport in polymer networks.\n                  <\/jats:p>","DOI":"10.1002\/adma.74571","type":"journal-article","created":{"date-parts":[[2026,8,17]],"date-time":"2026-08-17T08:31:59Z","timestamp":1786955519000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Bioinspired Hydrogen\u2010Bond Traps Enabling Ultrasensitive Temperature Sensing"],"prefix":"10.1002","volume":"38","author":[{"given":"Zhimin","family":"Lu","sequence":"first","affiliation":[{"name":"School of Materials Science and Engineering Tongji University  Shanghai China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yuhang","family":"Song","sequence":"additional","affiliation":[{"name":"School of Materials Science and Engineering Tongji University  Shanghai 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