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Polyphenols, a class of natural plant\u2010derived molecules, provide redox activity, multidentate interactions, and strong interfacial adhesion, making them versatile building blocks for bio\u2010derived agricultural systems. This review summarizes recent advances in the molecular design and multifunctional applications of polyphenol\u2010inspired materials across diverse agriculture sectors, including soil remediation, seed coating, nutrient delivery, crop protection, sensing, nitrification inhibition, and food preservation. It focuses on interfacial assembly, structure\u2013property relationships, and environmental interactions of polyphenol\u2010enabled materials, which collectively govern their performance from laboratory tests to field conditions. 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