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Inspired by the sense\u2010perceive\u2010act closed\u2010loop feedback of biological perspiration, we propose an autonomous thermal management strategy that encodes a first\u2010order solid\u2013liquid phase transition as a molecular logic gate. Within this phase\u2010change\u2010gated polymer network (Perspire X), the melting of polyethylene glycol (PEG) acts as a physical threshold. Surpassing this critical temperature triggers a macroscopic network arrangement, directly translating thermal sensing into an accelerated on\u2010demand water release. We define a logic\u2010gating figure of merit (LG\u2010FOM) of 2.62 to quantify this behavior, demonstrating the discretized and switchable regulation of coupled mass and heat transport channels. Consequently, the material exhibits non\u2010linear cooling amplification, achieving a 20.8\u2010fold extension in effective cooling duration and a 13.5\u00b0C temperature drop compared with traditional phase\u2010transition cooling materials. Furthermore, it demonstrates robust mechanical integrity alongside an exceptional thermal buffering capacity that effectively buffers the simulated pulsed thermal fluctuations under the tested conditions. Transcending traditional passive heat sinks, this phase\u2010transition\u2010gated transport mechanism outlines a scalable, materials\u2010level thermodynamic programming strategy for next\u2010generation electronics and intelligent energy systems.<\/jats:p>","DOI":"10.1002\/adma.74685","type":"journal-article","created":{"date-parts":[[2026,8,17]],"date-time":"2026-08-17T12:03:00Z","timestamp":1786968180000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Bio\u2010Inspired Phase\u2010Transition Logic Gates for Autonomous Thermal Management"],"prefix":"10.1002","volume":"38","author":[{"given":"Yabi","family":"Yang","sequence":"first","affiliation":[{"name":"State Key Laboratory of New Textile Materials and Advanced Processing, Research Center for Intelligent Fibre Devices and Equipment, Hubei Engineering Research Center For Biomaterials and Medical Protective Materials, Hubei Key Laboratory of Material Chemistry 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