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Misfit layered chalcogenides, which combine square and hexagonal lattices of rocksalt monochalcogenides and transition\u2010metal dichalcogenides, provide a platform to explore how incommensurability and explicit symmetry breaking impact collective electronic phases. Here we use low\u2010temperature scanning tunneling microscopy\/spectroscopy to probe the misfit compounds (MS)\n                    <jats:sub>1+\u03b4<\/jats:sub>\n                    TaS\n                    <jats:sub>2<\/jats:sub>\n                    with M = Pb, Sn and track how the misfit interface reshapes the electronic ground state of the embedded 1H\u2010TaS\n                    <jats:sub>2<\/jats:sub>\n                    monolayers. High\u2010resolution STM imaging and Fourier analysis reveal that the charge\u2010density wave (CDW) is incommensurate and exhibits spatially inhomogeneous, short\u2010range correlations. Strikingly, the CDW exhibits a pronounced and anisotropic response to the uniaxial moir\u00e9 potential imposed by the misfit layer: its coherence lengths and ordering wavevectors become inequivalent, demonstrating a strong nonlinear coupling between the intrinsic CDW instability and the symmetry\u2010breaking moir\u00e9 field. First\u2010principles\u2010informed multiscale modeling suggests that this reorganization arises from the combined effect of interlayer charge transfer and the spatially anisotropic energy landscape introduced by the misfit interface. In contrast, superconductivity is comparatively insensitive to the moir\u00e9, revealing a uniform, single full\u2010gap consistent with s\u2010wave pairing. Our results establish heterosymmetry stacking as a route to engineer correlated states in van der Waals materials.\n                  <\/jats:p>","DOI":"10.1002\/adma.74730","type":"journal-article","created":{"date-parts":[[2026,8,28]],"date-time":"2026-08-28T11:14:08Z","timestamp":1787915648000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Moir\u00e9\u2010Induced Symmetry Breaking of Charge Order in van der Waals Heterostructures"],"prefix":"10.1002","volume":"38","author":[{"ORCID":"https:\/\/orcid.org\/0009-0003-8395-4917","authenticated-orcid":false,"given":"Sandra","family":"Sajan","sequence":"first","affiliation":[{"name":"Donostia International Physics Center (DIPC) San Sebasti\u00e1n Spain"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0009-6554-6198","authenticated-orcid":false,"given":"Laura","family":"P\u00e4tzold","sequence":"additional","affiliation":[{"name":"I. Institute of Theoretical Physics University of Hamburg Hamburg Germany"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0002-2865-8800","authenticated-orcid":false,"given":"Tarushi","family":"Agarwal","sequence":"additional","affiliation":[{"name":"Department of Physics Indian Institute of Science Education and Research Bhopal  Bhopal India"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0008-4043-3595","authenticated-orcid":false,"given":"Clara","family":"Pfister","sequence":"additional","affiliation":[{"name":"I. Institute of Theoretical Physics University of Hamburg Hamburg Germany"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-4407-0081","authenticated-orcid":false,"given":"Haojie","family":"Guo","sequence":"additional","affiliation":[{"name":"Donostia International Physics Center (DIPC) San Sebasti\u00e1n Spain"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0001-3297-5238","authenticated-orcid":false,"given":"Sisheng","family":"Duan","sequence":"additional","affiliation":[{"name":"Donostia International Physics Center (DIPC) San Sebasti\u00e1n Spain"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-7090-3895","authenticated-orcid":false,"given":"P. V.","family":"Sruthibhai","sequence":"additional","affiliation":[{"name":"Centro de F\u00edsica de Materiales (CSIC\u2010UPV\/EHU)  San Sebasti\u00e1n Spain"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Mariana","family":"Rossi","sequence":"additional","affiliation":[{"name":"Max Planck Institute For the Structure and Dynamics of Matter  Hamburg Germany"},{"name":"Yusuf Hamied Department of Chemistry University of Cambridge  Cambridge UK"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-3552-0677","authenticated-orcid":false,"given":"Maria N.","family":"Gastiasoro","sequence":"additional","affiliation":[{"name":"Donostia International Physics Center (DIPC) San Sebasti\u00e1n Spain"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-4257-2651","authenticated-orcid":false,"given":"Sara","family":"Barja","sequence":"additional","affiliation":[{"name":"Donostia International Physics Center (DIPC) San Sebasti\u00e1n Spain"},{"name":"Centro de F\u00edsica de Materiales (CSIC\u2010UPV\/EHU)  San Sebasti\u00e1n Spain"},{"name":"Dept. Polymers and Advanced Materials University of the Basque Country (UPV\/EHU)  San Sebasti\u00e1n Spain"},{"name":"Ikerbasque, Basque Foundation for Science  Bilbao Spain"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-2548-231X","authenticated-orcid":false,"given":"Ravi P.","family":"Singh","sequence":"additional","affiliation":[{"name":"Department of Physics Indian Institute of Science Education and Research Bhopal  Bhopal India"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-5579-2231","authenticated-orcid":false,"given":"Tim","family":"Wehling","sequence":"additional","affiliation":[{"name":"I. 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