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Herein, a unique gel electrolyte with precise atomic\u2010level regulation of Zn\n                    <jats:sup>2+<\/jats:sup>\n                    migration is developed through incorporating Sn single\u2010atoms (SAs)\u2010loaded carbon fibers (CFs) into the polyacrylamide (PAM) matrix (PAM\/CFs@Sn) for building stable Zn anodes. The CFs fillers are introduced into the PAM gel electrolyte, which can promote more uniform Zn\n                    <jats:sup>2+<\/jats:sup>\n                    flux and charge distribution, thereby alleviating electric\u2010field heterogeneity. Meanwhile, the atomic\u2010level zincophilic Sn SAs sites offer abundant and uniform active centers to lower the Zn\n                    <jats:sup>2+<\/jats:sup>\n                    migration energy barrier, thereby promoting regular and planar Zn deposition. These combined advantages of the PAM\/CFs@Sn gel electrolyte enable Zn anodes to achieve stable cycling up to 3740\u00a0h at 0.5\u00a0mA cm\n                    <jats:sup>\u22122<\/jats:sup>\n                    , a high Zn\n                    <jats:sup>2+<\/jats:sup>\n                    transference number of 0.89 and an average coulombic efficiency of 99.5% over 1480\u00a0h, etc. Overall, this work provides a reliable atomic\u2010level zinc chemistry regulating strategy of gel electrolytes toward durable Zn anodes and beyond.\n                  <\/jats:p>","DOI":"10.1002\/adma.74734","type":"journal-article","created":{"date-parts":[[2026,8,20]],"date-time":"2026-08-20T14:04:57Z","timestamp":1787234697000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":4,"title":["Atomic\u2010Level Regulating Zinc Chemistry by Sn Single\u2010Atom\/Carbon\u2010Fibers Armed Gel Electrolyte for Highly Reversible Zinc Anode"],"prefix":"10.1002","volume":"38","author":[{"given":"Zeyu","family":"Yan","sequence":"first","affiliation":[{"name":"Department of Polymeric Materials &amp; Engineering College of Materials &amp; Metallurgy Guizhou University  Guiyang China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Song","family":"Yang","sequence":"additional","affiliation":[{"name":"Department of Polymeric Materials &amp; Engineering College of Materials &amp; Metallurgy Guizhou University  Guiyang China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Fusheng","family":"Luo","sequence":"additional","affiliation":[{"name":"Department of Polymeric Materials &amp; Engineering College of Materials &amp; Metallurgy Guizhou University  Guiyang China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jinlong","family":"Zhang","sequence":"additional","affiliation":[{"name":"Department of Polymeric Materials &amp; Engineering College of Materials &amp; Metallurgy 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