{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,8,29]],"date-time":"2026-08-29T04:17:50Z","timestamp":1787977070147,"version":"build-2784847793"},"reference-count":85,"publisher":"Wiley","license":[{"start":{"date-parts":[[2026,8,28]],"date-time":"2026-08-28T00:00:00Z","timestamp":1787875200000},"content-version":"vor","delay-in-days":0,"URL":"http:\/\/onlinelibrary.wiley.com\/termsAndConditions#vor"},{"start":{"date-parts":[[2026,8,28]],"date-time":"2026-08-28T00:00:00Z","timestamp":1787875200000},"content-version":"tdm","delay-in-days":0,"URL":"http:\/\/doi.wiley.com\/10.1002\/tdm_license_1.1"}],"funder":[{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["52573229"],"award-info":[{"award-number":["52573229"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["52173205"],"award-info":[{"award-number":["52173205"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["52473171"],"award-info":[{"award-number":["52473171"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100003399","name":"Science and Technology Commission of Shanghai Municipality","doi-asserted-by":"publisher","award":["25ZR1401213"],"award-info":[{"award-number":["25ZR1401213"]}],"id":[{"id":"10.13039\/501100003399","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100003399","name":"Science and Technology Commission of Shanghai Municipality","doi-asserted-by":"publisher","award":["25DZ3001002"],"award-info":[{"award-number":["25DZ3001002"]}],"id":[{"id":"10.13039\/501100003399","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":["advanced.onlinelibrary.wiley.com"],"crossmark-restriction":true},"short-container-title":["Advanced Materials"],"abstract":"<jats:title>ABSTRACT<\/jats:title>\n                  <jats:p>\n                    Olefin\u2010linked covalent organic frameworks (\n                    <jats:italic>cc<\/jats:italic>\n                    COFs) have shown great advantages in the community since discovery. However, the synthesis of ccCOFs highly relies on unsaturated heteroatom\u2010involved segments (uSHS) to activate C\u2500H bond to produce carbanion and to further condense with aldehydes. Such electron\u2010withdrawing uSHS have long hindered the wide applications of ccCOFs in optoelectronic devices due to the strong electron\u2010withdrawing effect. In this work, we report a carbenium\u2010involved synthesis of\n                    <jats:italic>cc<\/jats:italic>\n                    COFs without uSHS\u2019 participating. As\u2010synthesized ionic\n                    <jats:italic>cc<\/jats:italic>\n                    COFs show good crystallinity and ultra\u2010narrow bandgap down to 1.03\u00a0eV without introducing complicated donor\u2010acceptor building blocks. Such\n                    <jats:italic>cc<\/jats:italic>\n                    COFs can also be directly synthesized as uniform films on different substrates, for example, glass, silicon wafer, Au, and so on. Most impressively, the device Au\/2DPPPV\u2010102\/Al exhibits 32 distinct conductance states under low\u2010voltage sweeps and each conductance state demonstrated excellent non\u2010volatility and could be maintained stably for over 5000 s, which are typical features of memristor. A convolutional neural network was implemented using a 32\u2010conductance\u2010state memristor array and applied to image recognition, yielding recognition accuracies exceeding 90% for five randomly selected images.\n                  <\/jats:p>","DOI":"10.1002\/adma.74807","type":"journal-article","created":{"date-parts":[[2026,8,29]],"date-time":"2026-08-29T03:41:54Z","timestamp":1787974914000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Olefin\u2010Linked Ionic Covalent Organic Frameworks with Carbenium Backbones for High\u2010Performance Neuromorphic Computing"],"prefix":"10.1002","author":[{"ORCID":"https:\/\/orcid.org\/0009-0002-5113-7835","authenticated-orcid":false,"given":"Kaiyue","family":"Jiang","sequence":"first","affiliation":[{"name":"State Key Laboratory of Synergistic Chem\u2010Bio Synthesis State Key Laboratory of Metal Matrix Composites Shanghai Key Laboratory of Electrical Insulation and Thermal Ageing School of Chemistry and Chemical Engineering Shanghai Jiao Tong University  Shanghai P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0004-1716-5853","authenticated-orcid":false,"given":"Yuhang","family":"Zhou","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Synergistic Chem\u2010Bio Synthesis State Key Laboratory of Metal Matrix Composites Shanghai Key Laboratory of Electrical Insulation and Thermal Ageing School of Chemistry and Chemical Engineering Shanghai Jiao Tong University  Shanghai P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xiaolu","family":"Wang","sequence":"additional","affiliation":[{"name":"School of Physical Science and Technology Shanghai Key Laboratory of Highresolution Electron Microscopy ShanghaiTech University  Shanghai P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Dongyu","family":"Li","sequence":"additional","affiliation":[{"name":"School of Physical Science and Technology Shanghai Key Laboratory of Highresolution Electron Microscopy ShanghaiTech University  Shanghai P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xiaowei","family":"Wang","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Synergistic Chem\u2010Bio Synthesis State Key Laboratory of Metal Matrix Composites Shanghai Key Laboratory of Electrical Insulation and Thermal Ageing School of Chemistry and Chemical Engineering Shanghai Jiao Tong University  Shanghai P. R. China"},{"name":"Zhiyuan College Shanghai Jiao Tong University  Shanghai P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Cunyi","family":"Lv","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Synergistic Chem\u2010Bio Synthesis State Key Laboratory of Metal Matrix Composites Shanghai Key Laboratory of Electrical Insulation and Thermal Ageing School of Chemistry and Chemical Engineering Shanghai Jiao Tong University  Shanghai P. R. China"},{"name":"Zhiyuan College Shanghai Jiao Tong University  Shanghai P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Lei","family":"Zhao","sequence":"additional","affiliation":[{"name":"Shanghai Key Laboratory of Intelligent Sensing and Detection Institute of Intelligent Sensing and Instruments East China University of Science and Technology  Shanghai P. R. 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China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-0879-412X","authenticated-orcid":false,"given":"Feng","family":"Qiu","sequence":"additional","affiliation":[{"name":"School of Chemical and Environmental Engineering Shanghai Institute of Technology  Shanghai P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-9949-7525","authenticated-orcid":false,"given":"Wai\u2010Yeung","family":"Wong","sequence":"additional","affiliation":[{"name":"Department of Applied Biology and Chemical Technology and Research Institute for Smart Energy The Hong Kong Polytechnic University, Hung Hom  Hong Kong P. R. China"},{"name":"The Hong Kong Polytechnic University Shenzhen Research Institute  Shenzhen P. R. 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China"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2026,8,28]]},"reference":[{"key":"e_1_2_7_2_1","doi-asserted-by":"crossref","first-page":"1166","DOI":"10.1126\/science.1120411","article-title":"Porous, crystalline, covalent organic frameworks","volume":"310","author":"C\u00f4t\u00e9 A. P.","year":"2005","journal-title":"Science"},{"key":"e_1_2_7_3_1","doi-asserted-by":"crossref","first-page":"705","DOI":"10.1038\/nature01650","article-title":"Reticular Synthesis and the Design of New Materials","volume":"423","author":"Yaghi O. M.","year":"2003","journal-title":"Nature"},{"key":"e_1_2_7_4_1","doi-asserted-by":"crossref","DOI":"10.1126\/science.aal1585","article-title":"The Atom, the Molecule, and the Covalent Organic Framework","volume":"355","author":"Diercks C. 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