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While initially explored to overcome the efficiency limit of single\u2010junction photovoltaics, SF is now recognized as a broader platform for engineering correlated excited states. Efficient triplet generation and spin\u2010correlated pairs create opportunities in photovoltaics, photodetection, photocatalysis, photon up\u2010conversion, quantum light sources, spin\u2013photon interfaces, and bioimaging. This Review summarizes the fundamental mechanisms, energetic requirements, and molecular design principles governing SF, together with the influence of supramolecular organization and external stimuli on its dynamics. Particular emphasis is placed on the multiscale relationships among molecular energetics, excited\u2010state character, molecular packing, triplet\u2010pair separation, triplet transport, and interfacial energy or charge transfer, which ultimately determine device performance. We further discuss recent advances in SF\u2010enabled optoelectronic and quantum applications. Despite rapid progress, major challenges remain in establishing a unified mechanistic framework, understanding SF in polymeric and disordered systems, and expanding the library of stable, high\u2010performance SF materials. Finally, we highlight future opportunities in machine\u2010learning\u2010assisted materials discovery, excited\u2010state engineering, and the integration of SF into next\u2010generation functional optoelectronic devices.<\/jats:p>","DOI":"10.1002\/adma.74838","type":"journal-article","created":{"date-parts":[[2026,8,31]],"date-time":"2026-08-31T13:44:07Z","timestamp":1788183847000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Singlet Fission as an Exciton\u2010Management Platform for Next\u2010Generation Optoelectronic Materials"],"prefix":"10.1002","author":[{"given":"Lijuan","family":"Xue","sequence":"first","affiliation":[{"name":"School of Physics and Electrical Engineering Linyi University  Linyi China"},{"name":"Department of Physics City University of Hong Kong  Hong Kong SAR 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