{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,10,27]],"date-time":"2026-10-27T12:33:39Z","timestamp":1793104419557,"version":"4.5.0"},"reference-count":49,"publisher":"Wiley","issue":"60","license":[{"start":{"date-parts":[[2026,9,2]],"date-time":"2026-09-02T00:00:00Z","timestamp":1788307200000},"content-version":"vor","delay-in-days":0,"URL":"http:\/\/creativecommons.org\/licenses\/by-nc-nd\/4.0\/"},{"start":{"date-parts":[[2026,9,2]],"date-time":"2026-09-02T00:00:00Z","timestamp":1788307200000},"content-version":"tdm","delay-in-days":0,"URL":"http:\/\/doi.wiley.com\/10.1002\/tdm_license_1.1"}],"content-domain":{"domain":["advanced.onlinelibrary.wiley.com"],"crossmark-restriction":true},"short-container-title":["Advanced Materials"],"published-print":{"date-parts":[[2026,10]]},"abstract":"<jats:title>ABSTRACT<\/jats:title>\n                  <jats:p>\n                    Efficient generation and control of spin\u2010polarized currents in semiconductors remain central challenges for spin\u2010based electronics, particularly due to impedance mismatch and the reliance on magnetic fields or ferromagnetic contacts. Here, we introduce a materials platform for spectrally programmable spin transport based on a van der Waals (vdW) heterostructure combining the antiferromagnetic semiconductor NiPS\n                    <jats:sub>3<\/jats:sub>\n                    with WSe\n                    <jats:sub>2<\/jats:sub>\n                    . In a p\u2013n diode architecture, circularly polarized excitation produces pronounced photoconductive resonances with spin\u2010polarization reaching 80% near the N\u00e9el temperature and persisting at \u224830% at room temperature. Remarkably, selected spectral bands retain their polarization sign across the magnetic phase transition, evidencing robust, spectrally protected spin\u2010polarized current generation. Polarization\u2010resolved photogalvanic measurements reveal a dominant circular injection\u2010current mechanism, confirming spin\u2010polarized carrier transport. First\u2010principles calculations show that an applied electric field induces interfacial hybridization and spin\u2010layer locking, giving rise to localized symmetry breaking and enhanced optical absorption while preserving global time\u2010reversal symmetry. These results establish spectral tuning of excitation as a new control knob for spin transport, enabling spin\u2010current generation without magnetic fields or polarization switching. Our findings position magnetic vdW heterostructures as a versatile platform for opto\u2010spintronic functionality and spectrally programmable spintronic devices.\n                  <\/jats:p>","DOI":"10.1002\/adma.74889","type":"journal-article","created":{"date-parts":[[2026,9,2]],"date-time":"2026-09-02T13:06:30Z","timestamp":1788354390000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Spectrally Programmable Spin\u2010Polarized Photocurrents in WSe\n                    <sub>2<\/sub>\n                    \u2013NiPS\n                    <sub>3<\/sub>\n                    Magnetic van der Waals Heterostructures"],"prefix":"10.1002","volume":"38","author":[{"ORCID":"https:\/\/orcid.org\/0000-0003-3001-9207","authenticated-orcid":false,"given":"Rajesh Kumar","family":"Yadav","sequence":"first","affiliation":[{"name":"Faculty of Engineering Institute for Nanotechnology and Advanced Materials Bar\u2010Ilan University  Ramat\u2010Gan Israel"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-9534-5391","authenticated-orcid":false,"given":"Michal","family":"Poplinger","sequence":"additional","affiliation":[{"name":"Faculty of Engineering Institute for Nanotechnology and Advanced Materials Bar\u2010Ilan University  Ramat\u2010Gan Israel"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Adi","family":"Levi","sequence":"additional","affiliation":[{"name":"Faculty of Engineering Institute for Nanotechnology and Advanced Materials Bar\u2010Ilan University  Ramat\u2010Gan Israel"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-8401-8838","authenticated-orcid":false,"given":"Adi","family":"Harchol","sequence":"additional","affiliation":[{"name":"Schulich Faculty of Chemistry Solid State Institute Russell Berrie Nanotechnology Institute Helen Diller Quantum Information Center Technion  Haifa Israel"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-1982-4002","authenticated-orcid":false,"given":"Nirman","family":"Chakraborty","sequence":"additional","affiliation":[{"name":"Schulich Faculty of Chemistry Solid State Institute Russell Berrie Nanotechnology Institute Helen Diller Quantum Information Center Technion  Haifa Israel"},{"name":"Eduard Zintl Institute of Inorganic and Physical Chemistry Technical University of Darmstadt  Darmstadt Germany"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-5033-1065","authenticated-orcid":false,"given":"Thomas","family":"Brumme","sequence":"additional","affiliation":[{"name":"Faculty of Chemistry and Food Chemistry Technische Universit\u00e4t Dresden  Dresden Germany"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-2379-6251","authenticated-orcid":false,"given":"Thomas","family":"Heine","sequence":"additional","affiliation":[{"name":"Faculty of Chemistry and Food Chemistry Technische Universit\u00e4t Dresden  Dresden Germany"},{"name":"Center For Advanced Systems Understanding CASUS HZDR  G\u00f6rlitz Germany"},{"name":"Department of Chemistry and ibs for Nanomedicine Yonsei University  Seoul Republic of Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-7387-7821","authenticated-orcid":false,"given":"Efrat","family":"Lifshitz","sequence":"additional","affiliation":[{"name":"Schulich Faculty of Chemistry Solid State Institute Russell Berrie Nanotechnology Institute Helen Diller Quantum Information Center Technion  Haifa Israel"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-1091-5661","authenticated-orcid":false,"given":"Doron","family":"Naveh","sequence":"additional","affiliation":[{"name":"Faculty of Engineering Institute for Nanotechnology and Advanced Materials Bar\u2010Ilan University  Ramat\u2010Gan Israel"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2026,9,2]]},"reference":[{"key":"e_1_2_9_2_1","doi-asserted-by":"publisher","DOI":"10.1146\/annurev\u2010conmatphys\u2010070909\u2010104123"},{"key":"e_1_2_9_3_1","doi-asserted-by":"publisher","DOI":"10.1126\/science.1065389"},{"key":"e_1_2_9_4_1","doi-asserted-by":"publisher","DOI":"10.1103\/RevModPhys.76.323"},{"key":"e_1_2_9_5_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41699\u2010025\u201000546\u20104"},{"key":"e_1_2_9_6_1","doi-asserted-by":"publisher","DOI":"10.1007\/978-981-16-0069-2"},{"key":"e_1_2_9_7_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41567-018-0051-x"},{"key":"e_1_2_9_8_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41928\u2010024\u201001167\u20103"},{"key":"e_1_2_9_9_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41565\u2010021\u201000936\u2010x"},{"key":"e_1_2_9_10_1","doi-asserted-by":"publisher","DOI":"10.1038\/nphys2942"},{"key":"e_1_2_9_11_1","doi-asserted-by":"publisher","DOI":"10.1126\/science.1258122"},{"key":"e_1_2_9_12_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41565\u2010022\u201001115\u20102"},{"key":"e_1_2_9_13_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41566\u2010018\u20100204\u20106"},{"key":"e_1_2_9_14_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41586\u2010018\u20100631\u2010z"},{"key":"e_1_2_9_15_1","doi-asserted-by":"publisher","DOI":"10.1002\/inf2.12048"},{"key":"e_1_2_9_16_1","doi-asserted-by":"publisher","DOI":"10.1063\/5.0039979"},{"key":"e_1_2_9_17_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41563\u2010021\u201000968\u20107"},{"key":"e_1_2_9_18_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41567\u2010024\u201002618\u20106"},{"key":"e_1_2_9_19_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41586\u2010020\u20102520\u20105"},{"key":"e_1_2_9_20_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41467-021-27741-3"},{"key":"e_1_2_9_21_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41565\u2010021\u201000873\u20109"},{"key":"e_1_2_9_22_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41467\u2010025\u201065576\u20104"},{"key":"e_1_2_9_23_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41563\u2010023\u201001645\u20107"},{"key":"e_1_2_9_24_1","doi-asserted-by":"publisher","DOI":"10.1002\/adfm.202112750"},{"key":"e_1_2_9_25_1","doi-asserted-by":"publisher","DOI":"10.1002\/smll.202502479"},{"key":"e_1_2_9_26_1","doi-asserted-by":"publisher","DOI":"10.1098\/rspa.1934.0116"},{"key":"e_1_2_9_27_1","doi-asserted-by":"publisher","DOI":"10.1063\/1.1735965"},{"key":"e_1_2_9_28_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41699\u2010020\u201000188\u20108"},{"key":"e_1_2_9_29_1","doi-asserted-by":"publisher","DOI":"10.1016\/0031\u20108914(67)90062\u20106"},{"key":"e_1_2_9_30_1","doi-asserted-by":"publisher","DOI":"10.1063\/5.0107065"},{"key":"e_1_2_9_31_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41467\u2010021\u201025164\u20108"},{"key":"e_1_2_9_32_1","doi-asserted-by":"publisher","DOI":"10.1088\/0953-8984\/15\/20\/204"},{"key":"e_1_2_9_33_1","doi-asserted-by":"publisher","DOI":"10.1038\/nnano.2011.214"},{"key":"e_1_2_9_34_1","doi-asserted-by":"publisher","DOI":"10.1038\/ncomms8636"},{"key":"e_1_2_9_35_1","doi-asserted-by":"publisher","DOI":"10.1126\/science.aac6275"},{"key":"e_1_2_9_36_1","doi-asserted-by":"publisher","DOI":"10.1038\/nphys3105"},{"key":"e_1_2_9_37_1","doi-asserted-by":"publisher","DOI":"10.1038\/nphys2848"},{"key":"e_1_2_9_38_1","doi-asserted-by":"publisher","DOI":"10.2478\/v10155\u2010010\u20100086\u20108"},{"key":"e_1_2_9_39_1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.95.224430"},{"key":"e_1_2_9_40_1","doi-asserted-by":"publisher","DOI":"10.1021\/acs.nanolett.1c02188"},{"key":"e_1_2_9_41_1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.202107138"},{"key":"e_1_2_9_42_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41467\u2010023\u201040877\u20108"},{"key":"e_1_2_9_43_1","doi-asserted-by":"publisher","DOI":"10.1021\/acs.chemmater.4c02724"},{"key":"e_1_2_9_44_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.cpc.2009.06.022"},{"key":"e_1_2_9_45_1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevLett.77.3865"},{"key":"e_1_2_9_46_1","doi-asserted-by":"publisher","DOI":"10.1063\/1.4789814"},{"key":"e_1_2_9_47_1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevLett.124.146401"},{"key":"e_1_2_9_48_1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevMaterials.1.033803"},{"key":"e_1_2_9_49_1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevLett.115.036402"},{"key":"e_1_2_9_50_1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.101.235408"}],"container-title":["Advanced Materials"],"original-title":[],"language":"en","link":[{"URL":"https:\/\/advanced.onlinelibrary.wiley.com\/doi\/pdf\/10.1002\/adma.74889","content-type":"application\/pdf","content-version":"vor","intended-application":"text-mining"},{"URL":"https:\/\/advanced.onlinelibrary.wiley.com\/doi\/full-xml\/10.1002\/adma.74889","content-type":"application\/xml","content-version":"vor","intended-application":"text-mining"},{"URL":"https:\/\/advanced.onlinelibrary.wiley.com\/doi\/pdf\/10.1002\/adma.74889","content-type":"unspecified","content-version":"vor","intended-application":"similarity-checking"}],"deposited":{"date-parts":[[2026,10,27]],"date-time":"2026-10-27T11:46:58Z","timestamp":1793101618000},"score":1,"resource":{"primary":{"URL":"https:\/\/advanced.onlinelibrary.wiley.com\/doi\/10.1002\/adma.74889"}},"subtitle":[],"short-title":[],"issued":{"date-parts":[[2026,9,2]]},"references-count":49,"journal-issue":{"issue":"60","published-print":{"date-parts":[[2026,10]]}},"alternative-id":["10.1002\/adma.74889"],"URL":"https:\/\/doi.org\/10.1002\/adma.74889","archive":["Portico"],"relation":{},"ISSN":["0935-9648","1521-4095"],"issn-type":[{"value":"0935-9648","type":"print"},{"value":"1521-4095","type":"electronic"}],"subject":[],"published":{"date-parts":[[2026,9,2]]},"assertion":[{"value":"2026-04-11","order":0,"name":"received","label":"Received","group":{"name":"publication_history","label":"Publication History"}},{"value":"2026-08-26","order":2,"name":"accepted","label":"Accepted","group":{"name":"publication_history","label":"Publication History"}},{"value":"2026-09-02","order":3,"name":"published","label":"Published","group":{"name":"publication_history","label":"Publication History"}}],"article-number":"e74889"}}