{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,9,17]],"date-time":"2026-09-17T07:02:52Z","timestamp":1789628572852,"version":"build-2803163510"},"reference-count":58,"publisher":"Wiley","license":[{"start":{"date-parts":[[2026,9,16]],"date-time":"2026-09-16T00:00:00Z","timestamp":1789516800000},"content-version":"vor","delay-in-days":0,"URL":"http:\/\/onlinelibrary.wiley.com\/termsAndConditions#vor"},{"start":{"date-parts":[[2026,9,16]],"date-time":"2026-09-16T00:00:00Z","timestamp":1789516800000},"content-version":"tdm","delay-in-days":0,"URL":"http:\/\/doi.wiley.com\/10.1002\/tdm_license_1.1"}],"funder":[{"DOI":"10.13039\/501100004543","name":"China Scholarship Council","doi-asserted-by":"publisher","award":["202006630036"],"award-info":[{"award-number":["202006630036"]}],"id":[{"id":"10.13039\/501100004543","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":["advanced.onlinelibrary.wiley.com"],"crossmark-restriction":true},"short-container-title":["Advanced Materials"],"abstract":"<jats:title>ABSTRACT<\/jats:title>\n                  <jats:p>\n                    Emulating learning and memory functions of biological systems in soft, textile\u2010compatible materials remains challenging, particularly for artificial synapses that require both structural adaptability and reliable ionic dynamics. Existing artificial synaptic devices predominantly rely on membrane\u2010based or multilayered architectures, which complicate fabrication and limit scalability. Here, we report multiscale interfacial polyelectrolyte complexation (IPC) fibers fabricated via a one\u2010step interfacial process, enabling programmable fiber architectures with mechanical compliance and direct compatibility with smart textile platforms. The IPC fibers exhibit hierarchical structures spanning nanometer to micrometer length scales, promoting confined ionic transport and slow relaxation dynamics within flexible, thread\u2010like conductors. As a result, fiber\u2010based artificial synapses display pronounced short\u2010term plasticity with a tunable slow relaxation time constant (\n                    <jats:italic>\u03c4<\/jats:italic>\n                    <jats:sub>2<\/jats:sub>\n                    ), which spans several orders of magnitude and reaches up to 40 min owing to multiscale ion trapping and migration. Moreover, woven fiber arrays demonstrate both temporal and spatial summation of synaptic responses, enabling time\u2010dependent learning and pixel\u2010level memory encoding in IPC fiber arrays. The facile, environmentally benign fabrication strategy, combined with intrinsic structure\u2010function coupling in IPC fibers, establishes a versatile material and device platform for potential smart textiles, wearable neuromorphic systems, and adaptive fabrics.\n                  <\/jats:p>","DOI":"10.1002\/adma.74913","type":"journal-article","created":{"date-parts":[[2026,9,17]],"date-time":"2026-09-17T06:11:42Z","timestamp":1789625502000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Nonequilibrium Interfacial Complexation Fibers With Programmable Ionic Memory"],"prefix":"10.1002","author":[{"ORCID":"https:\/\/orcid.org\/0009-0008-7894-8877","authenticated-orcid":false,"given":"Ting","family":"Li","sequence":"first","affiliation":[{"name":"Graduate School of Science and Technology Kyoto Institute of Technology  Kyoto Japan"},{"name":"Institute for Functional Intelligent Materials National University of Singapore Singapore Singapore"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0005-1852-1618","authenticated-orcid":false,"given":"Jia Hui","family":"Bong","sequence":"additional","affiliation":[{"name":"Institute for Functional Intelligent Materials National University of Singapore Singapore Singapore"},{"name":"Department of Materials Science and Engineering National University of Singapore  Singapore Singapore"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-4781-5333","authenticated-orcid":false,"given":"Konstantin G.","family":"Nikolaev","sequence":"additional","affiliation":[{"name":"Institute for Functional Intelligent Materials National University of Singapore Singapore Singapore"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Hengrui","family":"Chen","sequence":"additional","affiliation":[{"name":"Institute for Functional Intelligent Materials National University of Singapore Singapore Singapore"},{"name":"Department of Materials Science and Engineering National University of Singapore  Singapore Singapore"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-3785-2218","authenticated-orcid":false,"given":"Xinyue","family":"Wen","sequence":"additional","affiliation":[{"name":"Institute for Functional Intelligent Materials National University of Singapore Singapore Singapore"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Panote","family":"Siriaraya","sequence":"additional","affiliation":[{"name":"Faculty of Information and Human Sciences Kyoto Institute of Technology  Kyoto Japan"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Noriaki","family":"Kuwahara","sequence":"additional","affiliation":[{"name":"Faculty of Information and Human Sciences Kyoto Institute of Technology  Kyoto 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V.","family":"Andreeva","sequence":"additional","affiliation":[{"name":"Institute for Functional Intelligent Materials National University of Singapore Singapore Singapore"},{"name":"Department of Materials Science and Engineering National University of Singapore  Singapore Singapore"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2026,9,16]]},"reference":[{"key":"e_1_2_9_2_1","doi-asserted-by":"crossref","first-page":"161","DOI":"10.1126\/science.adc9931","article-title":"Long\u2010Term Memory and Synapse\u2010Like Dynamics in Two\u2010Dimensional Nanofluidic Channels","volume":"379","author":"Robin P.","year":"2023","journal-title":"Science"},{"key":"e_1_2_9_3_1","doi-asserted-by":"crossref","first-page":"125","DOI":"10.1038\/s41578-018-0018-7","article-title":"Hydrogel Ionotronics","volume":"3","author":"Yang C.","year":"2018","journal-title":"Nature Reviews 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