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Here, a spectrally coordinated plasmonic\u2013photothermal\u2013photocatalytic architecture integrating Cu(II)\u2010grafted TiO\n                    <jats:sub>2<\/jats:sub>\n                    (CuT), yolk\u2013shell Au@SiO\n                    <jats:sub>2<\/jats:sub>\n                    (AuSi), and reduced graphene oxide sheets (GS) is presented for efficient mixed\u2010VOC mineralization under white light\u2010emitting diode (LED) illumination. Rather than acting as a simple multicomponent composite, this architecture couples partially overlapping but preferential spectral contributions across the LED spectrum: CuT drives visible\u2010light photocatalytic oxidation, AuSi contributes localized surface\u2010plasmon\u2010resonance\u2010induced electric\u2010field enhancement near CuT, and GS converts longer\u2010wavelength photons into localized heat to accelerate interfacial oxidation kinetics. Compared with CuT and binary controls, the composite enhances reactive oxygen species generation, CO\n                    <jats:sub>2<\/jats:sub>\n                    formation, and humidity tolerance. CuT\/AuSi\u2010GS enables near\u2010stoichiometric CO\n                    <jats:sub>2<\/jats:sub>\n                    formation during CH\n                    <jats:sub>3<\/jats:sub>\n                    CHO\/C\n                    <jats:sub>7<\/jats:sub>\n                    H\n                    <jats:sub>8<\/jats:sub>\n                    mixed\u2010VOC mineralization at 10 ppmv within 1\u00a0h and maintains over 80% CO\n                    <jats:sub>2<\/jats:sub>\n                    yield throughout 168\u00a0h of continuous\u2010flow operation at 2 ppmv. Chamber\u2010scale validation in a 64\u2010L reactor indicates the feasibility of VOC mineralization under a dedicated white LED source. Operando infrared spectroscopy traces stepwise oxidation of oxygenated and aromatic VOCs toward CO\n                    <jats:sub>2<\/jats:sub>\n                    , while wavelength\u2010dependent activity, spectral\u2010overlap analysis, thermal profiling, complementary spectroscopy, and simulations support coordinated energy utilization and deep mineralization under indoor white LED illumination.\n                  <\/jats:p>","DOI":"10.1002\/adma.74944","type":"journal-article","created":{"date-parts":[[2026,9,9]],"date-time":"2026-09-09T04:31:00Z","timestamp":1788928260000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Spectrally Coordinated Plasmonic\u2013Photothermal Photocatalysts for Mineralization of Mixed Indoor VOCs Under White LED 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