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Bubble adhesion on electrode surfaces blocks active sites, while gas accumulation in the bulk electrolyte disrupts ionic transport, collectively degrading electrochemical performance and operational stability. Conventional bubble\u2010management strategies primarily accelerate bubble departure, whereas gas\u2010diffusion architectures can provide preferential pathways for direct gas removal at the reaction interface. Here, we introduce a multiphase\u2010orchestrated electrolyzer architecture that physically separates gas management from electrocatalysis by positioning a hollow, gas\u2010permeable bladder adjacent to a conventional fully wetted electrode. Upon contact with the gas\u2010venting layer, nascent bubbles experience a wettability\u2010induced Laplace\u2010pressure bias and are rapidly transferred into a dedicated gas conduit, truncating bubble growth while preserving liquid access to the electrode. This spatial division of function decouples gas evacuation from electrolyte replenishment without external pumping. Under identical conditions, the optimized RGT architecture achieves up to a 2.1\u2010fold enhancement in current density in polarization measurements. The resulting modular framework provides an independently tunable strategy for regulating gas\u2013liquid transport in water electrolysis and other gas\u2010evolving electrochemical systems.<\/jats:p>","DOI":"10.1002\/adma.75008","type":"journal-article","created":{"date-parts":[[2026,9,14]],"date-time":"2026-09-14T04:34:17Z","timestamp":1789360457000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Asymmetric Laplace Pressure\u2010Mediated Multiphase Transport Decoupling for High\u2010Current Density Water Splitting"],"prefix":"10.1002","author":[{"given":"Yingjie","family":"Ji","sequence":"first","affiliation":[{"name":"State Key Laboratory of Organic\u2010Inorganic Composites Beijing Advanced Innovation Center for Soft Matter Science and Engineering Beijing University of Chemical Technology  Beijing People's Republic of 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Engineering Beijing University of Chemical Technology  Beijing People's Republic of China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Guixi","family":"Wang","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Organic\u2010Inorganic Composites Beijing Advanced Innovation Center for Soft Matter Science and Engineering Beijing University of Chemical Technology  Beijing People's Republic of China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xiaoke","family":"Li","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Organic\u2010Inorganic Composites Beijing Advanced Innovation Center for Soft Matter Science and Engineering Beijing University of Chemical Technology  Beijing People's Republic of China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Weikun","family":"Ren","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Organic\u2010Inorganic Composites Beijing Advanced 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