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As the field is progressing from laboratory demonstrations toward practical applications in soft robotics and biomedical devices, it is moving beyond the simple, uniform deformations toward advanced spatially programmable properties and integrated functionalities. The design principles underlying these advances lie in heterogeneous integration, defined as the intentional spatial design of chemical, structural, or orientational differences across a unified LCE system, permitting precise programming of differentiated actuation directions, mechanical gradients, and sequential responsiveness unattainable in homogeneous LCEs. Heterogeneous integration pervades almost all advances in alignment techniques, network engineering, and device assembly. This review categorizes the diverse achievements into three hierarchical strategies: heterogeneity in orientation, heterogeneity in polymer network architecture, and heterogeneous modular assembly. We systematically summarize the mechanistic origins, achievable precision, and functional outputs of each approach. Furthermore, we outline future directions from discrete patterning to continuous gradients, from single\u2010dimensional to multidimensional integration, and from static programming to adaptive evolution. This review establishes a coherent conceptual blueprint to guide the rational design of next\u2010generation intelligent LCE systems.<\/jats:p>","DOI":"10.1002\/adma.75020","type":"journal-article","created":{"date-parts":[[2026,9,21]],"date-time":"2026-09-21T10:45:20Z","timestamp":1789987520000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Heterogeneous Integration: Design Principles for Advanced Liquid Crystal Elastomers With Spatially Programmable Properties and Functionalities"],"prefix":"10.1002","author":[{"given":"Yixuan","family":"Wang","sequence":"first","affiliation":[{"name":"Department of Chemistry The Key Laboratory of Bioorganic Phosphorus Chemistry &amp; Chemical Biology (Ministry of Education) Tsinghua University  Beijing China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Enjian","family":"He","sequence":"additional","affiliation":[{"name":"Department of Chemistry The Key Laboratory of Bioorganic Phosphorus Chemistry &amp; Chemical Biology (Ministry of Education) Tsinghua University  Beijing China"},{"name":"AVIC Composite Corporation Ltd  Beijing China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Guoli","family":"Wang","sequence":"additional","affiliation":[{"name":"Electric Power Research Institute China Southern Power Grid Co. Ltd  Guangzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-5950-0163","authenticated-orcid":false,"given":"Yen","family":"Wei","sequence":"additional","affiliation":[{"name":"Department of Chemistry The Key Laboratory of Bioorganic Phosphorus Chemistry &amp; Chemical Biology (Ministry of Education) Tsinghua University  Beijing China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-1363-6513","authenticated-orcid":false,"given":"Yan","family":"Ji","sequence":"additional","affiliation":[{"name":"Department of Chemistry The Key Laboratory of Bioorganic Phosphorus Chemistry &amp; Chemical Biology (Ministry of Education) Tsinghua University  Beijing 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