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Although heating\u2010assisted charging enables ultrafast charging at elevated temperatures (e.g., 65\u00b0C), it increases the risk of thermal runaway. Lowering the activation energy of interfacial Li\u2010ion transport could enable safer room\u2010temperature XFC, although effective approaches remain limited. Here, we demonstrate that an amorphous Li\n                    <jats:sub>3<\/jats:sub>\n                    PO\n                    <jats:sub>4<\/jats:sub>\n                    \u2010Li\n                    <jats:sub>2<\/jats:sub>\n                    SO\n                    <jats:sub>4<\/jats:sub>\n                    \u2010rich solid electrolyte interphase (SEI), formed through electrolyte design, regulates interfacial Li\u2010ion transport by simultaneously tailoring SEI chemistry and facilitating Li\n                    <jats:sup>+<\/jats:sup>\n                    desolvation, with the apparent activation energy reduced from 39.1 to 21.3\u00a0kJ mol\n                    <jats:sup>\u22121<\/jats:sup>\n                    . As a result, 51.6 Ah pouch cells acquire 208.7\u00a0Wh kg\n                    <jats:sup>\u22121<\/jats:sup>\n                    of energy within only 10.5 min at room temperature (25\u00b0C), representing state\u2010of\u2010the\u2010art fast\u2010charging performance. Furthermore, a 94\u00a0kWh battery pack (3P168S) assembled from 504 mass\u2010produced pouch cells was integrated into a commercial electric vehicle. The pack was charged from 5% to 85% state\u2010of\u2010charge in 11.77 min, delivering 36.0\u00a0km of driving distance per minute of charge, surpassing the XFC target for electric vehicles (32.2\u00a0km min\n                    <jats:sup>\u22121<\/jats:sup>\n                    ). This work establishes an activation\u2010energy regulation strategy through coordinated control of interfacial solvation and SEI chemistry, providing a practical pathway toward room\u2010temperature XFC batteries and design principles for next\u2010generation fast\u2010charging technologies.\n                  <\/jats:p>","DOI":"10.1002\/adma.75045","type":"journal-article","created":{"date-parts":[[2026,9,22]],"date-time":"2026-09-22T12:00:26Z","timestamp":1790078426000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Extreme\u2010Fast\u2010Charging Li\u2010Ion Batteries via Activation\u2010Energy Regulation With a Li\n                    <sub>3<\/sub>\n                    PO\n                    <sub>4<\/sub>\n                    \u2010Li\n                    <sub>2<\/sub>\n                    SO\n                    <sub>4<\/sub>\n                    \u2010Rich Solid Electrolyte Interphase"],"prefix":"10.1002","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-6317-5049","authenticated-orcid":false,"given":"Wenfeng","family":"Mao","sequence":"first","affiliation":[{"name":"Academy of Interdisciplinary Studies On Intelligent Molecules, Tianjin Key Laboratory of Structure and Performance for Functional Molecules College of Chemistry Tianjin Normal University  Tianjin China"},{"name":"Guangzhou Greater Bay Technology (GBT) Co., Ltd  Guangzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Huarong","family":"Xia","sequence":"additional","affiliation":[{"name":"Innovative Centre for Flexible Devices (iFLEX) School of Materials Science and Engineering Nanyang Technological University  Singapore Singapore"},{"name":"School of Mechanical Engineering and Automation Fuzhou University  Fuzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Feng","family":"Pei","sequence":"additional","affiliation":[{"name":"Guangzhou Greater Bay Technology (GBT) Co., Ltd  Guangzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zhipeng","family":"Hu","sequence":"additional","affiliation":[{"name":"Academy of Interdisciplinary Studies On Intelligent Molecules, Tianjin Key Laboratory of Structure and Performance for Functional Molecules College of Chemistry Tianjin Normal University  Tianjin China"},{"name":"Guangzhou Greater Bay Technology (GBT) Co., Ltd  Guangzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Liya","family":"Cai","sequence":"additional","affiliation":[{"name":"Guangzhou Greater Bay Technology (GBT) Co., Ltd  Guangzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xiangbo","family":"Tang","sequence":"additional","affiliation":[{"name":"Guangzhou Greater Bay Technology (GBT) Co., Ltd  Guangzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Guo","family":"Ai","sequence":"additional","affiliation":[{"name":"Tianjin International Joint Research Centre of Surface Technology For Energy Storage Materials College of Physics and Materials Science Tianjin Normal University  Tianjin China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-8118-6502","authenticated-orcid":false,"given":"Xian Jun","family":"Loh","sequence":"additional","affiliation":[{"name":"Institute of Materials Research and Engineering (IMRE), Agency for Science Technology and Research (A*STAR)  Singapore Singapore"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-3312-1664","authenticated-orcid":false,"given":"Xiaodong","family":"Chen","sequence":"additional","affiliation":[{"name":"Innovative Centre for Flexible Devices (iFLEX) School of Materials Science and Engineering Nanyang Technological University  Singapore Singapore"},{"name":"School of Electrical and Electronic Engineering Nanyang Technological University  Singapore Singapore"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xiangdong","family":"Huang","sequence":"additional","affiliation":[{"name":"Guangzhou Greater Bay Technology (GBT) Co., Ltd  Guangzhou China"},{"name":"School of Mechanical &amp; Automotive Engineering South China University of Technology  Guangzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2026,9,22]]},"reference":[{"key":"e_1_2_10_2_1","doi-asserted-by":"crossref","unstructured":"D.Howell et\u00a0al. 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