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Inspiration from nature and its translation into the design of the next generation of intelligent materials are now in the limelight of research, from fundamental science to technological applications. Liquid crystals (LCs) represent a class of stimuli\u2010responsive soft matter that can serve as a key building block for smart and intelligent material systems. Bridging LC responsiveness with nanoscale functionalities gives rise to intelligent nanocomposite LC materials, which facilitate advanced development in soft robotics, adaptive camouflage, and transformative optics. In this review, we provide a comprehensive review of recent developments of bioinspired intelligent nanocomposite materials with responsive LCs and their promising applications, including reinforced LC elastomer nanocomposites for bioinspired soft actuators with self\u2010sensing functions and built\u2010in self\u2010feedback; bioinspired chiral nanocomposites with responsive LCs for adaptive camouflage, chiral plasmonics, and circularly polarized luminescence; and bioinspired reconfigurable metasurfaces with responsive LCs for ultra\u2010thin adaptive metalenses, dynamic meta\u2010holographic displays, and advanced beam steering devices. This review provides new insights into fostering interdisciplinary advances spanning nanotechnology, optics, mechanics, chemistry, materials science, and device engineering.<\/jats:p>","DOI":"10.1002\/adma.75064","type":"journal-article","created":{"date-parts":[[2026,9,24]],"date-time":"2026-09-24T10:04:29Z","timestamp":1790244269000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Bioinspired Intelligent Nanocomposite Liquid Crystal Materials: From Soft Actuators and Adaptive Camouflage to Transformative Optics"],"prefix":"10.1002","author":[{"ORCID":"https:\/\/orcid.org\/0009-0007-4513-0641","authenticated-orcid":false,"given":"Ran","family":"Bi","sequence":"first","affiliation":[{"name":"School of Materials Science and Engineering Tianjin University  Tianjin China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Sensheng","family":"Chen","sequence":"additional","affiliation":[{"name":"School of 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