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Here, we present an adhesive hydrogel based on lignin\u2010mediated catechol chemistry and salt hydrate phase\u2010transition, which achieves synergistic enhancement of interfacial adhesion and cohesive strength upon 1\u00a0V electrostimulated crystallization. The hydrogel is soft and exhibits mild adhesion to various substrates in amorphous state. Electrostimulus\u2010induced phase\u2010transition realizes a significant increment of cohesive strength and boosts interfacial adhesion by up to 8\u201340 times (exceeding 3000 J m\n                    <jats:sup>\u22122<\/jats:sup>\n                    ) on skin. The adhesion\u2010enhancement mechanisms on different substrates are elucidated via multi\u2010scale experimental designs and molecular simulations. When the hydrogel is applied as the adhesive layer, the assembled elastomer sensing devices inherit the electrostimulus adhesion\u2010enhancement and shape\u2010memory properties, significantly improving signal transmission stability and motion\u2010interference resistance. This study offers a simple and versatile strategy for stimuli\u2010enhanced adhesives, deepens the understanding of phase\u2010transition regulated adhesion behaviors, and supports the development of large\u2010area flexible devices for intelligent robotics and human\u2010computer interactions.\n                  <\/jats:p>","DOI":"10.1002\/adma.75100","type":"journal-article","created":{"date-parts":[[2026,9,21]],"date-time":"2026-09-21T04:52:13Z","timestamp":1789966333000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Electrostimulus Phase\u2010Transition Mediated Robust Adhesive Hydrogels"],"prefix":"10.1002","author":[{"given":"Jinlai","family":"Shen","sequence":"first","affiliation":[{"name":"School of Chemistry and Chemical Engineering State Key Laboratory of Advanced Papermaking and Paper\u2010based Materials South China University of Technology  Guangzhou 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