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The idea that electrical capacitors can serve as working bodies in a refrigeration cycle implies that electricity can be directly harnessed, potentially enabling the development of miniature and portable refrigerators, and has therefore attracted considerable attention from both academia and industry. Poly(vinylidene fluoride) (PVDF)\u2010based fluoropolymers exhibit strong dipolar responses and have been extensively studied for EC devices. However, despite their exceptional flexibility, straightforward synthesis, self\u2010healing capability, and low breakdown risk, their relatively low polar entropy\u2010changes limit their refrigeration capacities in practical applications. Rationally designing an EC polymer considering its molecular\u2010scale structure, crystalline features, and interfacial effects remains a major, nontrivial challenge. This work systematically reviews recent advances in EC polymers and focuses on two fundamental points pivotal for enhancing the polar entropy change, that is the electrocaloric effect (ECE): increasing zero\u2010field entropy and reducing the energy barrier of dipolar switching to increase electric field responsiveness. Together, they form a high\u2010polar\u2010entropy strategy that shows the potential to approach the lower and upper bounds of polar entropy to maximize the ECE. 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