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Phosphor ceramics provide a robust all\u2010inorganic alternative, but their photothermal coupling mechanisms and cross\u2010scale design principles remain insufficiently summarized. Here, we review recent advances in phosphor ceramics with a particular focus on photothermal coupling in high\u2010flux light conversion. We establish a composition\u2010structure\u2010photothermal behavior\u2010device performance framework that connects activator ions, host chemistry, defects and grain boundaries with light absorption, scattering regulation, thermal\u2010transport pathways, and device\u2010level output. Recent advances in garnet\u2010based, multiphase, multicolor visible, and NIR phosphor ceramics are discussed, with emphasis on compositional regulation, ceramic processing, microstructure engineering, and LED\/LD integration. We clarify key relationships among transparency, absorption efficiency, scattering strength, thermal conductivity, interfacial thermal resistance, and luminescence saturation thresholds, which collectively determine high\u2010brightness reliability under extreme photon and heat loads. Emerging glassy composite interfaces are further highlighted for low\u2010temperature integration, heterogeneous packaging, and multimaterial coupling. Finally, we discuss machine learning as an enabling tool for candidate screening, processing\u2010window optimization, property prediction, and multi\u2010objective device design, offering guidance for next\u2010generation stable, intelligent light\u2010conversion materials.<\/jats:p>","DOI":"10.1002\/adma.75219","type":"journal-article","created":{"date-parts":[[2026,10,1]],"date-time":"2026-10-01T04:41:26Z","timestamp":1790829686000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["From Phosphor Ceramics to Intelligent Light\u2010Conversion Materials: High\u2010Flux Luminescence, Glassy Composite Interface, and Machine\u2010Learning\u2010Guided Design"],"prefix":"10.1002","author":[{"ORCID":"https:\/\/orcid.org\/0009-0006-0436-8031","authenticated-orcid":false,"given":"Xiaoqing","family":"Pei","sequence":"first","affiliation":[{"name":"College of Physics and Energy Fujian Normal University  Fuzhou P. R. 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China"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2026,9,30]]},"reference":[{"key":"e_1_2_14_2_1","doi-asserted-by":"publisher","DOI":"10.1063\/5.0053581"},{"key":"e_1_2_14_3_1","doi-asserted-by":"publisher","DOI":"10.1021\/accountsmr.2c00193"},{"key":"e_1_2_14_4_1","doi-asserted-by":"publisher","DOI":"10.1117\/1.OE.61.6.060901"},{"key":"e_1_2_14_5_1","doi-asserted-by":"publisher","DOI":"10.1002\/lpor.201600147"},{"key":"e_1_2_14_6_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41560\u2010025\u201001757\u20101"},{"key":"e_1_2_14_7_1","doi-asserted-by":"publisher","DOI":"10.1021\/cm8030768"},{"key":"e_1_2_14_8_1","doi-asserted-by":"publisher","DOI":"10.1002\/lpor.201700344"},{"key":"e_1_2_14_9_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41377\u2010020\u20100326\u20108"},{"key":"e_1_2_14_10_1","doi-asserted-by":"publisher","DOI":"10.1115\/1.4044359"},{"key":"e_1_2_14_11_1","doi-asserted-by":"publisher","DOI":"10.1007\/s40145\u2010021\u20100467\u20100"},{"key":"e_1_2_14_12_1","doi-asserted-by":"publisher","DOI":"10.1002\/lpor.202200553"},{"key":"e_1_2_14_13_1","doi-asserted-by":"publisher","DOI":"10.1002\/lpor.202402144"},{"key":"e_1_2_14_14_1","doi-asserted-by":"publisher","DOI":"10.1039\/C8TC01178H"},{"key":"e_1_2_14_15_1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.202514881"},{"key":"e_1_2_14_16_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.cej.2025.172531"},{"key":"e_1_2_14_17_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.cej.2025.160077"},{"key":"e_1_2_14_18_1","doi-asserted-by":"publisher","DOI":"10.1080\/09506608.2019.1565716"},{"key":"e_1_2_14_19_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.actamat.2021.116813"},{"key":"e_1_2_14_20_1","doi-asserted-by":"publisher","DOI":"10.1002\/lpor.201300048"},{"key":"e_1_2_14_21_1","doi-asserted-by":"publisher","DOI":"10.1364\/JOSAB.469715"},{"key":"e_1_2_14_22_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.ijheatmasstransfer.2019.118600"},{"key":"e_1_2_14_23_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.jmst.2023.04.038"},{"key":"e_1_2_14_24_1","doi-asserted-by":"publisher","DOI":"10.1149\/2.023302jss"},{"key":"e_1_2_14_25_1","doi-asserted-by":"publisher","DOI":"10.15541\/jim20200652"},{"key":"e_1_2_14_26_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.jeurceramsoc.2018.03.043"},{"key":"e_1_2_14_27_1","doi-asserted-by":"publisher","DOI":"10.1039\/C6TC03215J"},{"key":"e_1_2_14_28_1","doi-asserted-by":"publisher","DOI":"10.1039\/C9TC00506D"},{"key":"e_1_2_14_29_1","doi-asserted-by":"publisher","DOI":"10.1063\/1.4742896"},{"key":"e_1_2_14_30_1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.201907888"},{"key":"e_1_2_14_31_1","doi-asserted-by":"publisher","DOI":"10.1002\/adom.202002141"},{"key":"e_1_2_14_32_1","doi-asserted-by":"publisher","DOI":"10.1111\/jace.17672"},{"key":"e_1_2_14_33_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.ceramint.2020.11.140"},{"key":"e_1_2_14_34_1","doi-asserted-by":"publisher","DOI":"10.1039\/C6CS00551A"},{"key":"e_1_2_14_35_1","doi-asserted-by":"publisher","DOI":"10.1039\/C8TC03866J"},{"key":"e_1_2_14_36_1","doi-asserted-by":"publisher","DOI":"10.1557\/jmr.2014.229"},{"key":"e_1_2_14_37_1","doi-asserted-by":"publisher","DOI":"10.1039\/C9TC04637B"},{"key":"e_1_2_14_38_1","doi-asserted-by":"publisher","DOI":"10.3390\/molecules29061325"},{"key":"e_1_2_14_39_1","doi-asserted-by":"publisher","DOI":"10.1364\/OE.27.000872"},{"key":"e_1_2_14_40_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.ceramint.2020.04.101"},{"key":"e_1_2_14_41_1","doi-asserted-by":"publisher","DOI":"10.1063\/5.0077184"},{"key":"e_1_2_14_42_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.jeurceramsoc.2020.10.027"},{"key":"e_1_2_14_43_1","doi-asserted-by":"crossref","DOI":"10.1016\/j.matchar.2021.110883","article-title":"Al2O3\u2013Ce:YAG 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