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Achieving a discharge plateau\/average operating voltage exceeding 2.0\u00a0V typically requires charging voltages above 2.5\u00a0V; however, the limited electrochemical stability of water molecules in has thus far prevented purely aqueous zinc batteries from reaching this threshold. Here, we report an extreme water\u2010confinement strategy that elevates the oxygen evolution potential of water in a poly(acrylamide\u2010co\u2010hydroxypropyl acrylate) hydrogel electrolyte to 2.85\u00a0V versus Zn\/Zn\n                    <jats:sup>2+<\/jats:sup>\n                    , far beyond the theoretical value (\u223c1.58\u00a0V versus Zn\/Zn\n                    <jats:sup>2+<\/jats:sup>\n                    ). This remarkable enhancement originates from the synergistic effects of strong cation\u2013water coordination, TFSI\n                    <jats:sup>\u2212<\/jats:sup>\n                    \u2010induced water segregation, and extensive hydrogen bonding within the polymer network, which collectively suppress water activity. When coupled with a lithium nickel manganese oxide cathode, the hydrogel electrolyte enables a 2.8 V\u2010class Zn\u2013Li hybrid battery that delivers a record\u2010breaking average operating voltage\/discharge plateau of 2.35\u00a0V, far exceeding all previously reported purely aqueous zinc batteries. The battery further exhibits excellent mechanical robustness and directly powers a multifunctional wireless sensing monitoring of dynamic pressure, finger movement, muscle activity, speech, and full\u2010body motion. This work provides a viable pathway toward ultrahigh\u2010voltage aqueous zinc batteries for next\u2010generation wearable and intelligent electronic systems.\n                  <\/jats:p>","DOI":"10.1002\/adma.75221","type":"journal-article","created":{"date-parts":[[2026,10,4]],"date-time":"2026-10-04T07:50:36Z","timestamp":1791100236000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Stabilizing Water Molecules in Hydrogel Electrolytes Enables 2.8 V\u2010Class Purely Aqueous Zn\u2013Li Hybrid Batteries"],"prefix":"10.1002","author":[{"given":"Meng","family":"Li","sequence":"first","affiliation":[{"name":"Interdisciplinary Research Center for Sustainable Energy Science and Engineering (IRC4SE2), School of Chemical Engineering Zhengzhou University  Zhengzhou P. R. 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